Deaktivierungsprozesse in isolierten aromatischen Heterocyclen und Pyrenen: = Deactivation processes in isolated aromatic heterocycles and pyrenes
Gespeichert in:
| Beteilige Person: | |
|---|---|
| Format: | Hochschulschrift/Dissertation Buch |
| Sprache: | Deutsch |
| Veröffentlicht: |
Würzburg
2017
|
| Schlagwörter: | |
| Links: | http://d-nb.info/1148787283/04 https://nbn-resolving.org/urn:nbn:de:bvb:20-opus-155445 http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030142710&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| Umfang: | xii, 239 Seiten Illustrationen, Diagramme 30 cm |
Internformat
MARC
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| 100 | 1 | |a Schmitt, Hans-Christian |d ca. 21. Jh. |e Verfasser |0 (DE-588)1151832367 |4 aut | |
| 245 | 1 | 0 | |a Deaktivierungsprozesse in isolierten aromatischen Heterocyclen und Pyrenen |b = Deactivation processes in isolated aromatic heterocycles and pyrenes |c vorgelegt von Hans-Christian Schmitt aus Bad Neustadt an der Saale |
| 246 | 1 | 1 | |a Deactivation processes in isolated aromatic heterocycles and pyrenes |
| 264 | 1 | |a Würzburg |c 2017 | |
| 300 | |a xii, 239 Seiten |b Illustrationen, Diagramme |c 30 cm | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 502 | |b Dissertation |c Julius-Maximilians-Universität Würzburg |d 2017 | ||
| 546 | |a Zusammenfassung in deutscher und englischer Sprache | ||
| 650 | 0 | 7 | |a Massenspektrometrie |0 (DE-588)4037882-2 |2 gnd |9 rswk-swf |
| 650 | 0 | 7 | |a Angeregter Zustand |0 (DE-588)4142423-2 |2 gnd |9 rswk-swf |
| 650 | 0 | 7 | |a Pyren |0 (DE-588)4176461-4 |2 gnd |9 rswk-swf |
| 650 | 0 | 7 | |a Heteroaromaten |0 (DE-588)4159717-5 |2 gnd |9 rswk-swf |
| 650 | 0 | 7 | |a Laserspektroskopie |0 (DE-588)4034620-1 |2 gnd |9 rswk-swf |
| 653 | |a time-resolved spectroscopy | ||
| 655 | 7 | |0 (DE-588)4113937-9 |a Hochschulschrift |2 gnd-content | |
| 689 | 0 | 0 | |a Heteroaromaten |0 (DE-588)4159717-5 |D s |
| 689 | 0 | 1 | |a Pyren |0 (DE-588)4176461-4 |D s |
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| 689 | 0 | |5 DE-604 | |
| 776 | 0 | 8 | |i Erscheint auch als |n Online-Ausgabe |o urn:nbn:de:bvb:20-opus-155445 |a Schmitt, Hans-Christian |t Deaktivierungsprozesse in isolierten aromatischen Heterocyclen und Pyrenen |d Würzburg : Universität Würzburg, 2017 |h Online-Ressource |
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Datensatz im Suchindex
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| _version_ | 1821935804527673344 |
| adam_text | INHALTSVERZEICHNIS
ABKUERZUNGSVERZEICHNIS VII
PUBLIKATIONSLISTE XI
1 EINLEITUNG 1
2 THEORETISCHE GRUNDLAGEN 5
2.1 S PEKTROSKOPIE IN D E R G A S P H A S E
...........................................................................
5
2.1.1 M O LEKULARSTRAHL-S P EK TRO SK O P IE
.............................................................. 5
2.1 .2 R ESO N AN ZV ERSTAERK TE M E H R P H O TO N E N IO N IS A TIO N
.................................... 7
2.1 .3 F ITFUNKTION Z U R E RM ITTLU N G D E R L EB EN SD AU ER AN G
EREG TER Z U STAE N D E 10
2.2 PHOTOPHYSIKALISCHE P R O Z E S S E
.................................................................................
10
2.2.1 A BSORPTION
....................................................................................................
11
2.2 .2 S TRAH LU N G SLO SE UE B E R G AE N G E
.......................................................................
12
2.2.2.1 THEORIE D ER STRA H LU N G SLO SE N UE B E RG AE N G E
................................. 14
2 .2 .2 .2 INNERE U M W ANDLUNG ( I C )
..........................................................
15
2 .2 .2 .3 IN TERSY STEM C ROSSING ( I S C )
....................................................... 16
2 .2 .2 .4 K ONISCHE D U RC H SC H N E ID U N G ( C I )
.............................................
18
2.3 C LU S TE R E X P E R IM E N TE
.................................................................................................
18
2.3.1 C LU S TE R B ILD U N G
..............................................................................................
18
2 .4 E X C I M E R E
.......................................................... 20
3 EXPERIMENTELLER AUFBAU 25
3.1 P IK O SEK U N D EN L ASERSYSTEM FUE R G A SP H ASEN -S P EK TRO SK O
P IE
.......................
25
3.1.1 N D:Y L F -L ASER
......................................................
25
3.1 .2 H ARM ONISCHE E I N H E I T
.................................................................................
27
3.1 .3 O P TISCH ER P A RA M E TRISCH E R G E N E R A T O R
.................................................... 27
3.2 G A S P H A S E N -A P P A RA TU
R..............................................................................................
29
3.3 A UFBAU U N D IN B ETRIEB N AH M E D E R N E U E N IM AG IN G -G ASP
H ASEN -A P P ARATU R . 30
3.3.1 V A K U U M K O M P O N E N TE N
.................................................................................
30
3 .3 .2 V A K U U M E RZ E U G U N G
..........................................................................
32
3 .3 .3 M OLEKULARSTRAHLQUELLE . . .
.
...............................................................
36
3 .3 .4 V U V -Z E LLE
.......................................................................................................
37
3 .3 .5 E LEK TRO N ISCH E B AUTEILE
..............................................................................
38
3.3.5.1 IO N E N O P TIK
........................................................................................
38
3 .3 .5 .2 D E TE K TO R
...........................................................................................
41
3 .3 .5 .3 S P A N N U N G S Q U E LLE N
........................................................................
4 4
3 .3 .5 .4 H O C H S P A N N U N G S -T RA N S IS TO RS C H A LTE R
.......................................
4 4
3 .3 .5 .5 D E LA Y -G E N E RA TO RE N
........................................................................
45
3 .3 .5 .6 S TRO M M O N ITO R
.................................................................................
45
3 .3 .6 IN B E TRIE B N A H M E D E R A P P A RA TU R
..............................................................
46
3.3.6.1 P Y R ID IN
...............................................................................................
46
3 .3 .6 .2 B RO M B E N Z O
L.....................................................................................
4 8
3 .3 .6 .3 A NILIN
...............................................................................................
51
3 .3 .7 ZEITLICHE S TE U E RU N G D ES E X P E R IM E N TS
....................................................
54
3 .3.7.1 T O F -M O D U S
.....................................................................................
54
3 .3 .7 .2 K A TIO N E N -IM A G IN G -M O D U S
...................
54
3 .3 .7 .3 E LEK TRO N EN -IM AG IN G -M O D U S
.......................................................
55
4 1,8-NAPHTHALIMID 57
4.1 S TA N D D E R F O R S C H U N G
..............................................................................
58
4.2 E R G E B N I S S E
..................................................................................................................
59
4.2.1 T HEO RETISCH E B ESCH REIB U N G D E R LAGE AN G EREG TER E LEK
TRO N ISCH ER Z U
S TAE N D E VON N I
..................................................................................................
59
4 .2 .2 M A S S E N S P E K TRU M
...........................................................................................
60
4 .2 .3 W E LLE N LAE N G E N -S C A N
........................................................................................
61
4 .2 .4 ZEITAUFGELOESTE E X P E RIM E N TE
........................................................................
64
4 .2 .5 S IM U LATIO N EN Z U R B ESCH REIB U N G DER M O LE K UE LD Y N
A M IK
.....................
66
4.3 Z U SA M M E N FA SSU N G U N D D IS K U S S IO N
....................................................................
69
4 .4 N A P H TH A LIM ID -D IM E
R..................................................................................................
72
5 N-HETEROCYCLISCHE C ARBENE 77
5.1 E IG EN SCH AFTEN VON N H C S
..........................................................................
78
5.2 S TA N D D E R F O R S C H U N G
...............................................................................................
79
5.3 1,3-DI- TE RT-B U TY L-IM ID A Z O LIN -2 -Y LID E N
.................................................................
80
5.3.1 R EC H N U N G E N Z U R LAGE D E R ELEK TRO N ISCH AN G EREG TEN
Z U STAE N D E . . . 80
5 .3 .2 M A S S E N S P E K TR U M
...........................................................................................
81
5 .3 .3 W E LLE N LAE N G E N -S C A N
........................................................................................
82
5 .3 .4 Z EITAUFGELOESTE E X P E RIM E N TE
........................................................................
83
5 .3 .5 1,3-DI- TE RT-B U TY L-IM ID A Z O LO N
....................................................................
84
5.3.5.1 R ECH N U N G EN Z U R LAGE D E R AN G EREG TEN Z U S T AE N D E
................
86
5 .3 .5 .2 M A S S E N S P E K TRU M
...........................................................................
88
5 .3 .5 .3 I N F R A R O T- S P E K TR U M
........................................................................
89
5 .3 .5 .4 W E LLE N LAE N G E N -S C A N S
.................................................................... 90
5 .3 .5 .5 Z EITAUFGELOESTE E X P E RIM E N TE
.......................................................
93
5.4 Z U SA M M E N FASSU N G U N D D IS K U S S IO N
................................................................... 95
6 PYREN 99
6.1 S TA N D D E R F O R S C H U N G
..............................................................................................
100
6.2 T HEORETISCHE B ESCH REIB U N G D E R E X C IM E RB ILD U N G
.............................................. 102
6.2.1 S TRU K TU R U N D ANGEREGTE Z U STAE N D E D ES P Y RE N D IM E RS
..........................
102
6.3 E XPERIM ENTELLE E R G E B N I S S E
....................................................................................
107
6.3.1 M A S S E N S P E K T R E N
...........................................................................................
108
6.3.2 W E LLE N LAE N G E N -S C A N S
....................................................................................
109
6 .3 .3 ZEITAUFGELOESTE M E S S U N G E N
...........................................................................
111
6.4 N ICHTADIABATISCHE D YNAM IK S IM U LA TIO N E N
.......................................................
115
6.5 Z U SA M M E N FASSU N G U N D D IS K U S S IO N
.................................................................... 118
7 2-HYDROXYPYREN 121
7.1 E R G E B N I S S E
..........................................................................
123
7.1.1 T HEORETISCHE B ESCH REIB U N G D E R LAGE E LEK TRO N ISCH AN G
EREG TER Z U
STAE N D E IM 2 -H Y D RO X Y P Y RE N
.......................................................................
123
7.1.2 T HEORETISCHE B ESCHREIB U N G DES 2 -H Y D RO X Y P Y RE N D IM E
RS
................
125
7.1.3 M A S S E N S P E K TRU M
...........................................................................................
126
7.1 .4 W E LLE N LAE N G E N -S C A N S
....................................................................................
127
7.1.5 ZEITAUFGELOESTE E X P E RIM E N TE
.......................................................................
132
7.2 Z U SA M M E N FASSU N G U N D D IS K U S S IO N
.................................................................... 136
8 WEITERE AROMATISCHE HETEROCYCLEN 139
8.1 A T -M ETHYL-PHTHALIM
ID..............................................................................................
139
8.1.1 S TA N D D E R F O R S C H U N G
.................................................................................
140
8.1 .2 E RGEBNISSE
....................................................................................................
141
8.1.2.1 W E LLE N LAE N G E N -S C A N S
.................................................................... 141
8 .1 .2 .2 ZEITAUFGELOESTE E X P E RIM E N TE
.......................................................
146
8.1.3 Z U SA M M E N FASSU N G U N D D IS K U S S IO N
.......................................................
147
8.2 X A N TH O N
.........................................
148
8.2.1 S TA N D D E R F O R S C H U N G
.................................................................................
149
8.2.2 E RGEBNISSE
....................................................................................................
154
8.2.2.1 W ELLEN LAE N G E N -S C A N
.......................................................................
155
8.2 .2 .2 ZEITAUFGELOESTE E X P E RIM E N TE
.......................................................
155
8 .2 .3 Z U SA M M E N FASSU N G U N D D IS K U S S IO N
.......................................................
159
8.3 C H R O M O N
....................................................................................................................
162
8.3.1 S TA N D D E R F O R S C H U N G
..................................................................................
162
8 .3 .2 E RGEBNISSE
.....................................................................................................
163
8.3.2.1 W E LLE N LAE N G E N -S C A N
........................................................................
163
8 .3 .2 .2 ZEITAUFGELOESTE E X P E RIM E N TE
.......................................................
164
8 .3 .3 Z U SA M M E N FA SSU N G U N D D IS K U S S IO N
........................................................ 166
9 BENZOCYLCOBUTEN-1,2-DION 169
9.1 S TA N D D E R F O R S C H U N G
...............................................................................................
170
9.2 E XPERIM ENTELLES S E TU P
...........................................................................................
174
9.3 E R G E B N I S S E
..................................................................................................................
175
9.3.1 V OREXPERIM ENTE A N B E N Z O C Y C LO B U TE N -L,2 -D IO N
....................................
175
9 .3.1.1 U V /V IS - S P E K TR U M
........................................................................
175
9 .3 .1 .2 I R - S P E K T R U M
..................................................................................
176
9 .3 .2 R ECH N U N G EN ZU M B E N Z O C Y C LO B U TE N -L,2 -D IO N
............................................177
9 .3 .3 U V /IR -E X P E RIM E N TE
.....................................................................................
177
9.3.3.1 G RO U N D S TA TE B LEACH
.................................................................
177
9 .3 .3 .2 B IS K E TE N B ILD U N G
......................
179
9 .3 .3 .3 B ILDUNG W EITERER S P E Z I E S
........................................................... 181
9 .3 .4 U V /V IS -E X P E RIM E N
T.....................................................................................
182
9 .3 .5 A NALYSE D E R EXPERIM EN TELLEN D A T E N
.......................................................
184
9.3.5.1 G LOBALE A NALYSE
...........................................................................
185
9 .3 .5 .2 Z I E L A N A L Y S E
.....................................................................................
188
9 .4 Z U SA M M E N FASSU N G U N D D IS K U S S IO N
.....................................................................
189
10 ZUSAMMENFASSUNG 193
11 SUMMARY 197
LITERATURVERZEICHNIS 201
DANKSAGUNG
237
|
| any_adam_object | 1 |
| author | Schmitt, Hans-Christian ca. 21. Jh |
| author_GND | (DE-588)1151832367 |
| author_facet | Schmitt, Hans-Christian ca. 21. Jh |
| author_role | aut |
| author_sort | Schmitt, Hans-Christian ca. 21. Jh |
| author_variant | h c s hcs |
| building | Verbundindex |
| bvnumber | BV044746971 |
| classification_rvk | VE 5070 |
| collection | ebook |
| ctrlnum | (OCoLC)1135368277 (DE-599)DNB1148787283 |
| discipline | Chemie / Pharmazie |
| format | Thesis Book |
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"><subfield code="5">DE-604</subfield></datafield><datafield tag="776" ind1="0" ind2="8"><subfield code="i">Erscheint auch als</subfield><subfield code="n">Online-Ausgabe</subfield><subfield code="o">urn:nbn:de:bvb:20-opus-155445</subfield><subfield code="a">Schmitt, Hans-Christian</subfield><subfield code="t">Deaktivierungsprozesse in isolierten aromatischen Heterocyclen und Pyrenen</subfield><subfield code="d">Würzburg : Universität Würzburg, 2017</subfield><subfield code="h">Online-Ressource</subfield></datafield><datafield tag="856" ind1="4" ind2="2"><subfield code="m">B:DE-101</subfield><subfield code="q">application/pdf</subfield><subfield code="u">http://d-nb.info/1148787283/04</subfield><subfield code="3">Inhaltsverzeichnis</subfield></datafield><datafield tag="856" ind1="4" ind2="1"><subfield code="u">https://nbn-resolving.org/urn:nbn:de:bvb:20-opus-155445</subfield><subfield code="x">Resolving-System</subfield><subfield code="z">kostenfrei</subfield><subfield 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| genre | (DE-588)4113937-9 Hochschulschrift gnd-content |
| genre_facet | Hochschulschrift |
| id | DE-604.BV044746971 |
| illustrated | Illustrated |
| indexdate | 2024-12-20T18:10:36Z |
| institution | BVB |
| language | German |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-030142710 |
| oclc_num | 1135368277 |
| open_access_boolean | 1 |
| owner | DE-384 DE-473 DE-BY-UBG DE-703 DE-1051 DE-824 DE-29 DE-12 DE-91 DE-BY-TUM DE-19 DE-BY-UBM DE-1049 DE-92 DE-739 DE-898 DE-BY-UBR DE-355 DE-BY-UBR DE-706 DE-20 DE-1102 DE-860 DE-2174 |
| owner_facet | DE-384 DE-473 DE-BY-UBG DE-703 DE-1051 DE-824 DE-29 DE-12 DE-91 DE-BY-TUM DE-19 DE-BY-UBM DE-1049 DE-92 DE-739 DE-898 DE-BY-UBR DE-355 DE-BY-UBR DE-706 DE-20 DE-1102 DE-860 DE-2174 |
| physical | xii, 239 Seiten Illustrationen, Diagramme 30 cm |
| psigel | ebook |
| publishDate | 2017 |
| publishDateSearch | 2017 |
| publishDateSort | 2017 |
| record_format | marc |
| spellingShingle | Schmitt, Hans-Christian ca. 21. Jh Deaktivierungsprozesse in isolierten aromatischen Heterocyclen und Pyrenen = Deactivation processes in isolated aromatic heterocycles and pyrenes Massenspektrometrie (DE-588)4037882-2 gnd Angeregter Zustand (DE-588)4142423-2 gnd Pyren (DE-588)4176461-4 gnd Heteroaromaten (DE-588)4159717-5 gnd Laserspektroskopie (DE-588)4034620-1 gnd |
| subject_GND | (DE-588)4037882-2 (DE-588)4142423-2 (DE-588)4176461-4 (DE-588)4159717-5 (DE-588)4034620-1 (DE-588)4113937-9 |
| title | Deaktivierungsprozesse in isolierten aromatischen Heterocyclen und Pyrenen = Deactivation processes in isolated aromatic heterocycles and pyrenes |
| title_alt | Deactivation processes in isolated aromatic heterocycles and pyrenes |
| title_auth | Deaktivierungsprozesse in isolierten aromatischen Heterocyclen und Pyrenen = Deactivation processes in isolated aromatic heterocycles and pyrenes |
| title_exact_search | Deaktivierungsprozesse in isolierten aromatischen Heterocyclen und Pyrenen = Deactivation processes in isolated aromatic heterocycles and pyrenes |
| title_full | Deaktivierungsprozesse in isolierten aromatischen Heterocyclen und Pyrenen = Deactivation processes in isolated aromatic heterocycles and pyrenes vorgelegt von Hans-Christian Schmitt aus Bad Neustadt an der Saale |
| title_fullStr | Deaktivierungsprozesse in isolierten aromatischen Heterocyclen und Pyrenen = Deactivation processes in isolated aromatic heterocycles and pyrenes vorgelegt von Hans-Christian Schmitt aus Bad Neustadt an der Saale |
| title_full_unstemmed | Deaktivierungsprozesse in isolierten aromatischen Heterocyclen und Pyrenen = Deactivation processes in isolated aromatic heterocycles and pyrenes vorgelegt von Hans-Christian Schmitt aus Bad Neustadt an der Saale |
| title_short | Deaktivierungsprozesse in isolierten aromatischen Heterocyclen und Pyrenen |
| title_sort | deaktivierungsprozesse in isolierten aromatischen heterocyclen und pyrenen deactivation processes in isolated aromatic heterocycles and pyrenes |
| title_sub | = Deactivation processes in isolated aromatic heterocycles and pyrenes |
| topic | Massenspektrometrie (DE-588)4037882-2 gnd Angeregter Zustand (DE-588)4142423-2 gnd Pyren (DE-588)4176461-4 gnd Heteroaromaten (DE-588)4159717-5 gnd Laserspektroskopie (DE-588)4034620-1 gnd |
| topic_facet | Massenspektrometrie Angeregter Zustand Pyren Heteroaromaten Laserspektroskopie Hochschulschrift |
| url | http://d-nb.info/1148787283/04 https://nbn-resolving.org/urn:nbn:de:bvb:20-opus-155445 http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030142710&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT schmitthanschristian deaktivierungsprozesseinisoliertenaromatischenheterocyclenundpyrenendeactivationprocessesinisolatedaromaticheterocyclesandpyrenes AT schmitthanschristian deactivationprocessesinisolatedaromaticheterocyclesandpyrenes |