Confocal and near-field optical microscopy and spectroscopy of organic materials: from molecules to thin solid films
Gespeichert in:
| Beteilige Person: | |
|---|---|
| Format: | Hochschulschrift/Dissertation Buch |
| Sprache: | Englisch |
| Veröffentlicht: |
2012
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| Schlagwörter: | |
| Links: | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025484959&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| Beschreibung: | Enth. dtsprachige Zsfassung |
| Umfang: | IV, 140 S. Ill., graph. Darst. |
Internformat
MARC
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| 003 | DE-604 | ||
| 005 | 20130109 | ||
| 007 | t| | ||
| 008 | 130108s2012 xx ad|| m||| 00||| eng d | ||
| 035 | |a (OCoLC)843424697 | ||
| 035 | |a (DE-599)BSZ376366060 | ||
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| 100 | 1 | |a Wang, Xiao |e Verfasser |4 aut | |
| 245 | 1 | 0 | |a Confocal and near-field optical microscopy and spectroscopy of organic materials |b from molecules to thin solid films |c vorgelegt von Xiao Wang |
| 264 | 1 | |c 2012 | |
| 300 | |a IV, 140 S. |b Ill., graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 500 | |a Enth. dtsprachige Zsfassung | ||
| 502 | |a Tübingen, Univ., Diss., 2012 | ||
| 655 | 7 | |0 (DE-588)4113937-9 |a Hochschulschrift |2 gnd-content | |
| 856 | 4 | 2 | |m DNB Datenaustausch |q application/pdf |u http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025484959&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |3 Inhaltsverzeichnis |
| 943 | 1 | |a oai:aleph.bib-bvb.de:BVB01-025484959 | |
Datensatz im Suchindex
| _version_ | 1819266131184058368 |
|---|---|
| adam_text | IMAGE 1
CONTENTS
1 INTRODUCTION 1
2 THEORETICAL FOUNDATIONS A N D E X P E R I M E N T A L M E T H O D S 5
2.1 OPTICAL MICROSCOPY A T THE NANOSCALE 6
2.1.1 FAR-FIELD AND NEAR-FIELD 6
2.1.2 OPTICAL RESOLUTION 7
2.1.3 FAR-FIELD OPTICAL MICROSCOPY 9
2.1.4 NEAR-FIELD OPTICAL MICROSCOPY 11
2.2 PLASMONICS AND ENHANCED RAMAN SCATTERING 13
2.2.1 PLASMON AND SURFACE PLASMON POLARITONS 13
2.2.2 LOCALIZED SURFACE PLASMON 16
2.2.3 RAMAN AND SURFACE ENHANCED RAMAN SCATTERING 17
2.2.3.1 THEORY OF RAMAN SCATTERING 17
2.2.3.2 SURFACE ENHANCED RAMAN SCATTERING (SERS) 21
2.2.4 T I P ENHANCED RAMAN SCATTERING 22
2.3 PARABOLIC MIRROR ASSISTED OPTICAL MICROSCOPY 24
2.3.1 LASER MODES 24
2.3.1.1 FUNDAMENTAL GAUSSIAN MODE 24
2.3.1.2 RADIAL AND AZIMUTHAL MODE 25
2.3.2 T H E OPTICAL PATH 26
2.3.3 FIELD DISTRIBUTION OF T H E FOCUS 27
2.3.3.1 THEORETICAL SIMULATION 27
2.3.3.2 EXPERIMENTAL MEASUREMENT 28
I
HTTP://D-NB.INFO/103244469X
IMAGE 2
C O N T E N T S
2.3.4 TIP PREPARATION 30
2.3.5 SAMPLE TIP DISTANCE CONTROL 30
2.3.6 ALIGNMENT OF THE TIP IN THE FOCUS . . 33
2.3.7 SPECTROSCOPIC IMAGING 33
3 P O L Y M E R FULLERENE B L E N D FILMS FOR SOLAR CELL APPLICATIONS 3
5
3.1 ORGANIC POLYMER FULLERENE SOLAR CELLS : 36
3.1.1 PRINCIPLES 36
3.1.2 POLYMER AND FULLERENE BLEND FILM 37
3.1.3 MORPHOLOGY CHARACTERIZATION 39
3.2 IMAGING CHEMICAL CONTRAST OF P3HT:PCBM BLEND FILMS 41
3.2.1 P3HT:PCBM BLEND FILMS 41
3.2.2 CONFOCAL SPECTROSCOPIC MAPPING 42
3.2.3 NEAR-FIELD SPECTROSCOPIC MAPPING 46
3.2.3.1 FILMS SUBJECTED TO 30 MIN. OF ANNEALING 46
3.2.3.2 FILMS SUBJECTED T O 5 MIN. OF ANNEALING 49
3.2.4 SUMMARY 51
3.3 NANOSCALE PHASE SEPARATION OF C-PCPDTBT:PCBM BLEND FILM 53
3.3.1 C-PCPDTBT:PCBM BLEND FILM 53
3.3.2 P L AND RAMAN SPECTRA 53
3.3.3 CONFOCAL SPECTROSCOPIC MAPPING 56
3.3.4 NEAR-FIELD SPECTROSCOPIC MAPPING 58
3.3.5 SUMMARY 61
3.4 SI-PCPDTBT:PCBM BLEND FILMS _ 64
3.4.1 BLEND FILM PERPARATION 64
3.4.2 PHOTOLUMINESCENCE AND RAMAN SPECTROSCOPY 64
3.4.3 SUMMARY 68
3.5 PHOTO-DEGRADATION OF POLYMER FULLERENE BLEND FILM 69
3.5.1 PHOTO-DEGRADATION OF P3HT:PCBM BLEND FILMS 69
3.5.2 PHOTO-DEGRADATION OF C-PCPDTBT:PCBM BLEND FILMS 71
3.5.3 SUMMARY 76
II
IMAGE 3
C O N T E N T S
4 X E R S S T U D I E S O F ALIZARIN-TIOJ A N D ALIZARIN-AU C O M P L E
X 7 7
4.1 T1O2 SURFACE STATES AND INTERFACIAL ELECTRONIC COUPLING WITH
ALIZARIN 78
4.1.1 INTERFACIAL ELECTRON TRANSFER 78
4.1.2 TIC 2 AND ALIZARIN SYSTEM 80
4.1.3 IMAGING OF SINGLE TICVSURFACE STATES AND INTERFACIAL ELECTRONIC
COUPLING 80
4.1.4 SUMMARY 87
4.2 SERS A N D TERS STUDIES OF ALIZARIN ADSORBED ON A U 88
4.2.1 EXPERIMENTAL 89
4.2.2 ALIZARIN WITH AU NANOPARTICLE 90
4.2.3 SERS OF ALIZARIN WITH THE AU GRID 91
4.2.4 RAMAN CALCULATIONS OF THE ALIZARIN-AU COMPLEX 93
4.2.5 SERS AND TERS OF ALIZARIN WITH ROUGH AU FILM 95
4.2.5.1 CONFOCAL SURFACE-ENHANCED RAMAN IMAGING 95
4.2.5.2 TIP-ENHANCED RAMAN IMAGING 97
4.2.6 SUMMARY - 100
5 OPTICAL PROPERTIES O F P E N P F P A N D T H E B L E N D FILMS 1 0 1
5.1 MORPHOLOGY CORRELATED R A M A N SPECTROSCOPIC STUDIES OF PENTACENE
FILMS . . . . 102
5.1.1 EXPERIMENTAL 102
5.1.2 PENTACENE THIN FILM 103
5.1.3 CONFOCAL OPTICAL IMAGES AND SPECTROSCOPY 103
5.1.4 MORPHOLOGY CORRELATED RAMAN SPECTROSCOPY 105
5.1.5 SUMMARY 108
5.2 OPTICAL IMAGING AND SPECTROSCOPY OF P F P AND P F P : P E N BLEND
FILMS 109
5.2.1 EXPERIMENTAL 109
5.2.2 CONFOCAL AND NEAR-FIELD OPTICAL STUDIES OF P F P FILMS 109
5.2.3 TOPOGRAPHY RELATED CONFOCAL OPTICAL STUDIES OF P F P : P E N (3:1)
BLEND
FILMS 114
5.2.4 CONFOCAL OPTICAL STUDIES OF P F P : P E N (1:3) BLEND FILMS 116
5.2.5 SUMMARY 118
III
IMAGE 4
C O N T E N T S
6 CONCLUSION 1 1 9
BIBLIOGRAPHY 1 2 3
ABBREVIATIONS 1 3 5
ACKNOWLEDGMENT 1 3 7
PUBLICATIONS 1 3 9
I V
|
| any_adam_object | 1 |
| author | Wang, Xiao |
| author_facet | Wang, Xiao |
| author_role | aut |
| author_sort | Wang, Xiao |
| author_variant | x w xw |
| building | Verbundindex |
| bvnumber | BV040658153 |
| ctrlnum | (OCoLC)843424697 (DE-599)BSZ376366060 |
| dewey-full | 502.82 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 502 - Miscellany |
| dewey-raw | 502.82 |
| dewey-search | 502.82 |
| dewey-sort | 3502.82 |
| dewey-tens | 500 - Natural sciences and mathematics |
| discipline | Allgemeine Naturwissenschaft |
| format | Thesis Book |
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| genre_facet | Hochschulschrift |
| id | DE-604.BV040658153 |
| illustrated | Illustrated |
| indexdate | 2024-12-20T16:19:53Z |
| institution | BVB |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-025484959 |
| oclc_num | 843424697 |
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| physical | IV, 140 S. Ill., graph. Darst. |
| publishDate | 2012 |
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| spellingShingle | Wang, Xiao Confocal and near-field optical microscopy and spectroscopy of organic materials from molecules to thin solid films |
| subject_GND | (DE-588)4113937-9 |
| title | Confocal and near-field optical microscopy and spectroscopy of organic materials from molecules to thin solid films |
| title_auth | Confocal and near-field optical microscopy and spectroscopy of organic materials from molecules to thin solid films |
| title_exact_search | Confocal and near-field optical microscopy and spectroscopy of organic materials from molecules to thin solid films |
| title_full | Confocal and near-field optical microscopy and spectroscopy of organic materials from molecules to thin solid films vorgelegt von Xiao Wang |
| title_fullStr | Confocal and near-field optical microscopy and spectroscopy of organic materials from molecules to thin solid films vorgelegt von Xiao Wang |
| title_full_unstemmed | Confocal and near-field optical microscopy and spectroscopy of organic materials from molecules to thin solid films vorgelegt von Xiao Wang |
| title_short | Confocal and near-field optical microscopy and spectroscopy of organic materials |
| title_sort | confocal and near field optical microscopy and spectroscopy of organic materials from molecules to thin solid films |
| title_sub | from molecules to thin solid films |
| topic_facet | Hochschulschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025484959&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT wangxiao confocalandnearfieldopticalmicroscopyandspectroscopyoforganicmaterialsfrommoleculestothinsolidfilms |