Activation of nitrogen oxides by supported noble metal catalysts: structure-activity relationships
Gespeichert in:
| Beteilige Person: | |
|---|---|
| Format: | Hochschulschrift/Dissertation Buch |
| Sprache: | Englisch |
| Veröffentlicht: |
München
Verl. Dr. Hut
2010
|
| Ausgabe: | 1. Aufl. |
| Schriftenreihe: | Anorganische Chemie
|
| Schlagwörter: | |
| Links: | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=020867820&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| Umfang: | 116 S. Ill., graph. Darst. |
| ISBN: | 9783868536775 |
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| 100 | 1 | |a Beyer, Hans |e Verfasser |4 aut | |
| 245 | 1 | 0 | |a Activation of nitrogen oxides by supported noble metal catalysts |b structure-activity relationships |c Hans Beyer |
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| 264 | 1 | |a München |b Verl. Dr. Hut |c 2010 | |
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Datensatz im Suchindex
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| DE-BY-TUM_katkey | 1752503 |
| DE-BY-TUM_location | Mag |
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| adam_text | IMAGE 1
TABLE OF CONTENTS
1 ACTIVATION OF NITROGEN OXIDES BY NOBLE METAL CATALYSTS 1
1.1 ORIGINS AND EFFECTS OF NITROGEN OXIDES 2
1.2 CHALLENGES IN THE ACTIVATION OF NITROGEN OXIDES BY NOBLE METAL
CATALYSTS....6
1.3 AIM AND MOTIVATION OF THE PRESENT WORK 8
2 NO» REMOVAL BY RHODIUM CATALYSTS SUPPORTED ON CARBON NANOTUBES:
EVIDENCE FOR THE STOICHIOMETRIC REDUCTION OF NO X BY THE CARBON SUPPORT
9
2.1 STATE OF THE ART 10
2.1.1 DIRECT DECOMPOSITION OF NO X BY RHODIUM CATALYSTS 10
2.1.2 CARBON MATERIALS IN HETEROGENEOUS CATALYSIS 11
2.1.3 NO REMOVAL BY NOBLE METAL CATALYSTS SUPPORTED ON CARBON 12
2.2 AIM AND MOTIVATION 12
2.3 CATALYTIC ACTIVITY 13
2.4 REACTION MECHANISM 23
2.5 STRUCTURAL DEVELOPMENT OF CATALYST MATERIALS 24
2.6 IMPACT OF EXCESS OXYGEN ON CATALYTIC ACTIVITY 25
2.7 CONCLUSIONS 26
3 DECOMPOSITION OF NITROUS OXIDE BY RHODIUM CATALYSTS:
EFFECT OF RHODIUM PARTICLE SIZE AND METAL OXIDE SUPPORT 27
3.1 ACID-BASE PROPERTIES OF METAL OXIDE SURFACES AND THEIR ROLE IN
CATALYSIS... 28
3.2 STATE OF THE ART: DECOMPOSITION OF N2O BY RHODIUM CATALYSTS 36
3.3 AIM AND MOTIVATION 40
3.4 CATALYTIC ACTIVITY 40
3.4.1 GENERAL COMPARISON 41
3.4.2 IMPACT OF EXCESS OXYGEN 43
3.4.3 IMPACT OF THE RHODIUM PRECURSOR 44
3.5 CATALYST CHARACTERIZATION 45
3.5.1 RHODIUM PARTICLE SIZE 45
3.5.2 REDOX PROPERTIES OF RHODIUM PARTICLES 48
3.6 DISCUSSION OF STRUCTURE-ACTIVITY RELATIONSHIPS 49
3.7 CONCLUSIONS 51
BIBLIOGRAFISCHE INFORMATIONEN HTTP://D-NB.INFO/1008935654
DIGITALISIERT DURCH
IMAGE 2
TABLE OF CONTENTS
4 INFLUENCE OF LIGHT ON THE ACTIVATION OF NO BY SUPPORTED NOBLE METAL
CATALYSTS 53
4.1 MATERIALS, METHODS AND APPLICATIONS OF HETEROGENEOUS
PHOTOCATALYSIS....54
4.2 PREPARATION OF MESOPOROUS TRANSITION METAL OXIDES 58
4.2.1 STATE OF THE ART 58
4.2.2 AIM AND MOTIVATION 60
4.2.3 PREPARATION AND CHARACTERIZATION OF
TITANIUM/TANTALUM MIXED OXIDES 61
4.2.4 PREPARATION AND CHARACTERIZATION OF
DOPED TITANIUM AND TANTALUM OXIDES 64
4.2.5 CONCLUSIONS 68
4.3 PHOTOASSISTED REDUCTION OF NO WITH PROPANE
BY SUPPORTED SILVER CATALYSTS 69
4.3.1 STATE OF THE ART 69
4.3.2 AIM AND MOTIVATION OF THE PHOTOASSISTED CATALYSIS APPROACH 70
4.3.3 DESIGN OF AN UV/VIS IRRADIATED TUBE FURNACE
AND A FLUIDIZED BED PHOTOREACTOR 71
4.3.4 CATALYTIC ACTIVITY 73
4.3.5 CATALYST CHARACTERIZATION 75
4.3.6 STRUCTURE-ACTIVITY RELATIONSHIPS AND EFFECTS OF UV/VIS
IRRADIATION.. 79
4.3.7 CONCLUSIONS 80
5 SUMMARY 81
6 ZUSAMMENFASSUNG 85
IMAGE 3
TABLE OF CONTENTS
7 EXPERIMENTAL 89
7.1 CATALYST PREPARATION 90
7.1.1 TEMPLATE SYNTHESIS OF MESOPOROUS TRANSITION METAL OXIDES 90
7.1.1.1 LIGAND ASSISTED TEMPLATING METHOD 90
7.1.1.2 NEUTRAL SURFACTANT TEMPLATING METHOD 92
7.1.2 CATALYST PREPARATION BY INCIPIENT WETNESS IMPREGNATION 94
7.2 ANALYTICAL METHODS 96
7.2.1 QUANTITATIVE GAS ANALYSIS 96
7.2.1.1 FOURIER TRANSFORM INFRARED SPECTROSCOPY 96
7.2.1.2 MICRO GAS CHROMATOGRAPHY 97
7.2.2 SORPTION BASED AND TEMPERATURE PROGRAMMED ANALYSIS 98
3.2.2.1 N 2 PHYSISORPTION 99
3.2.2.2 CO PULSE CHEMISORPTION 99
3.2.2.3 TEMPERATURE PROGRAMMED REDUCTION 100
7.2.3 X-RAY DIFFRACTION 100
7.2.4 TRANSMISSION ELECTRON MICROSCOPY 101
7.2.5 ELEMENTAL ANALYSIS 101
7.2.6 ELECTRON PARAMAGNETIC RESONANCE SPECTROSCOPY 101
7.3 CATALYTIC MEASUREMENTS 102
7.3.1 INSTRUMENTAL SETUP FOR CATALYTIC ACTIVITY TESTS 102
7.3.2 CONSTRUCTION OF AN UV/VIS IRRADIATED TUBE FURNACE 103
7.3.3 CATALYTIC TEST PROCEDURES 104
8 APPENDIX 105
8.1 LIST OF PUBLICATIONS 106
8.2 CONFERENCE CONTRIBUTIONS 106
9 REFERENCES 109
|
| any_adam_object | 1 |
| author | Beyer, Hans |
| author_facet | Beyer, Hans |
| author_role | aut |
| author_sort | Beyer, Hans |
| author_variant | h b hb |
| building | Verbundindex |
| bvnumber | BV036952798 |
| classification_tum | CHE 167d CHE 331d CHE 366d CHE 372d CHE 373d CHE 376d |
| ctrlnum | (OCoLC)706965170 (DE-599)BVBBV036952798 |
| dewey-full | 628.53 |
| dewey-hundreds | 600 - Technology (Applied sciences) |
| dewey-ones | 628 - Sanitary engineering |
| dewey-raw | 628.53 |
| dewey-search | 628.53 |
| dewey-sort | 3628.53 |
| dewey-tens | 620 - Engineering and allied operations |
| discipline | Chemie / Pharmazie Physik Bauingenieurwesen |
| edition | 1. Aufl. |
| format | Thesis Book |
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| genre_facet | Hochschulschrift |
| id | DE-604.BV036952798 |
| illustrated | Illustrated |
| indexdate | 2024-12-20T14:45:17Z |
| institution | BVB |
| isbn | 9783868536775 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-020867820 |
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| owner_facet | DE-91 DE-BY-TUM DE-12 |
| physical | 116 S. Ill., graph. Darst. |
| publishDate | 2010 |
| publishDateSearch | 2010 |
| publishDateSort | 2010 |
| publisher | Verl. Dr. Hut |
| record_format | marc |
| series2 | Anorganische Chemie |
| spellingShingle | Beyer, Hans Activation of nitrogen oxides by supported noble metal catalysts structure-activity relationships Trägerkatalysator (DE-588)4185817-7 gnd Aktivierung Chemie (DE-588)4141761-6 gnd Stickstoffoxide (DE-588)4057516-0 gnd Edelmetall (DE-588)4013531-7 gnd Struktur-Aktivitäts-Beziehung (DE-588)4183784-8 gnd |
| subject_GND | (DE-588)4185817-7 (DE-588)4141761-6 (DE-588)4057516-0 (DE-588)4013531-7 (DE-588)4183784-8 (DE-588)4113937-9 |
| title | Activation of nitrogen oxides by supported noble metal catalysts structure-activity relationships |
| title_auth | Activation of nitrogen oxides by supported noble metal catalysts structure-activity relationships |
| title_exact_search | Activation of nitrogen oxides by supported noble metal catalysts structure-activity relationships |
| title_full | Activation of nitrogen oxides by supported noble metal catalysts structure-activity relationships Hans Beyer |
| title_fullStr | Activation of nitrogen oxides by supported noble metal catalysts structure-activity relationships Hans Beyer |
| title_full_unstemmed | Activation of nitrogen oxides by supported noble metal catalysts structure-activity relationships Hans Beyer |
| title_short | Activation of nitrogen oxides by supported noble metal catalysts |
| title_sort | activation of nitrogen oxides by supported noble metal catalysts structure activity relationships |
| title_sub | structure-activity relationships |
| topic | Trägerkatalysator (DE-588)4185817-7 gnd Aktivierung Chemie (DE-588)4141761-6 gnd Stickstoffoxide (DE-588)4057516-0 gnd Edelmetall (DE-588)4013531-7 gnd Struktur-Aktivitäts-Beziehung (DE-588)4183784-8 gnd |
| topic_facet | Trägerkatalysator Aktivierung Chemie Stickstoffoxide Edelmetall Struktur-Aktivitäts-Beziehung Hochschulschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=020867820&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT beyerhans activationofnitrogenoxidesbysupportednoblemetalcatalystsstructureactivityrelationships |
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