Physical chemistry of electrolyte solutions: modern aspects
Gespeichert in:
| Beteiligte Personen: | , , |
|---|---|
| Format: | Buch |
| Sprache: | Deutsch |
| Veröffentlicht: |
Darmstadt
Steinkopff
1998
New York Springer |
| Schriftenreihe: | Topics in physical chemistry
5 |
| Schlagwörter: | |
| Links: | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=008003362&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| Beschreibung: | Literaturangaben |
| Umfang: | XVII, 401 S. graph. Darst. |
| ISBN: | 3798510768 |
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Datensatz im Suchindex
| _version_ | 1819244963790061568 |
|---|---|
| adam_text | J. M. G. BARTHEL H. KRIENKE W. KUNZ TOPICS IN PHYSICAL CHEMISTRY 5
PHYSICAL CHEMISTRY OF ELECTROLYTE SOLUTIONS EDITED BY H. BAUMGAERTEL E.
U. FRANCK W. GRUENBEIN ON BEHALF OF DEUTSCHE BUNSEN-GESELLSCHAFT FUER
PHYSIKALISCHE CHEMIE MODERN ASPECTS 9 STEINKOPFF DARMSTADT ** SPRINGER
CONTENTS PREFACE V 1 ION ASSOCIATION AND SOLVATION IN ELECTROLYTE
SOLUTIONS 1 1.1 CLASSIFICATION OF SOLVENTS AND ELECTROLYTES 1 1.1.1
SOLVENT PARAMETERS AND SOLVENT CLASSES 1 1.1.2 ION CLASSES 4 1.1.3
IONIZING SOLVATION REACTIONS 14 1.2 THERMODYNAMICS OF ELECTROLYTE
SOLUTIONS 15 1.3 TWO PARTICLE INTERACTIONS IN THE VACUUM 21 1.3.1
ATTRACTIVE POTENTIALS OF SPATIALLY FIXED IONS AND DIPOLES 21 1.3.2
ANGLE-AVERAGED POTENTIALS AND VAN DER WAALS POTENTIAL 23 1.3.3
SELF-ENERGIES 24 1.3.4 COMPLETE INTERMOLECULAR PAIR POTENTIALS 25 1.3.5
ELECTROSTATIC POTENTIALS AROUND PARTICLES WITH ARBITRARY INTRAMOLECULAR
CHARGE DISTRIBUTIONS 26 1.4 IONS AND MOLECULES IN HOMOGENEOUS DIELECTRIC
MEDIA 27 1.4.1 ION IN AN ELECTROLYTE SOLUTION 28 1.4.2 DIPOLE MOLECULE
IN A HOMOGENEOUS DIELECTRIC MEDIUM 29 1.4.3 REACTION FIELD 30 1.4.4
POLARIZATION IN GASES AND LIQUIDS 31 1.4.5 COMPLETE ION-ION INTERACTION
POTENTIALS IN SOLUTIONS 33 1.4.6 PARTICLE SIZE PARAMETERS 35 1.5
SOLVATION MODELS 40 1.5.1 IONS AND SOLVENT MOLECULES IN THE GAS PHASE 40
1.5.2 ION SOLVATION IN THE LIQUID PHASE 44 1.5.3 ION TRANSFER QUANTITIES
52 REFERENCES 53 2 TRANSPORT AND RELAXATION PHENOMENA IN ELECTROLYTE
SOLUTIONS .... 59 2.1 FLOWS AND CURRENTS 59 2.2 PRINCIPLES OF NORMAL
MODE ANALYSIS 62 2.3 DIFFUSION 65 2.3.1 CHEMICAL DIFFUSION OF A
COMPLETELY DISSOCIATED ELECTROLYTE 67 2.3.2 CHEMICAL DIFFUSION OF
ASSOCIATED ELECTROLYTES 68 2.4 CHARGE TRANSPORT 70 2.4.1 CHARGE FLOW IN
EXTERNAL ELECTRIC FIELDS 70 2.4.2 TRANSFERENCE NUMBERS AND SINGLE ION
CONDUCTIVITIES 72 XIV CONTENTS 2.4.3 APPARENT IONIC CHARGES 74 2.4.4
EMPIRICAL INVESTIGATION ON ELECTROLYTE CONDUCTIVITY 75 2.5 HYDRODYNAMIC
PROPERTIES OF ELECTROLYTE SOLUTIONS 80 2.5.1 VISCOSITY 80 2.5.2 BULK
VISCOSITY OF SOLVENTS AND ELECTROLYTE SOLUTIONS 82 2.5.3 SPHERICAL
PARTICLES IN A VISCOUS CONTINUUM 83 2.6 DIELECTRIC POLARIZATION 88 2.6.1
PHENOMENOLOGICAL ASPECTS 90 2.6.2 RESPONSE FUNCTIONS 93 2.6.3 MOLECULAR
CORRELATION FUNCTIONS 97 2.6.4 RELAXATION SPECTRA OF PURE LIQUIDS AND
THEIR MIXTURES 98 2.6.5 RELAXATION SPECTRA OF ELECTROLYTE SOLUTIONS 104
2.6.6 IONIC EQUILIBRIA IN ELECTROLYTE SOLUTIONS 108 2.7 REDOX REACTIONS
IN SOLUTION 110 2.8 ULTRASONIC ABSORPTION 113 REFERENCES 115 3
ELECTROLYTE SOLUTIONS AT LOW TO MODERATE CONCENTRATIONS 121 3.1
MOLECULAR DISTRIBUTION FUNCTIONS 121 3.2 CHEMICAL MODEL AT LOW
ELECTROLYTE CONCENTRATIONS 124 3.2.1 MEAN FORCE POTENTIAL 124 3.2.2 THE
ACTIVITY COEFFICIENT OF THE LCCM 127 3.2.3 THE ION-PAIR CONCEPT OF THE
LCCM 128 3.2.4 ELECTROLYTE SOLUTION PROPERTIES ON THE LCCM LEVEL 130 3.3
THERMODYNAMIC PROPERTIES OF ELECTROLYTE SOLUTIONS 131 3.3.1 ACTIVITY
COEFFICIENTS AND OSMOTIC COEFFICIENTS 131 3.3.2 FITTING EQUATIONS FOR
ACTIVITY AND OSMOTIC COEFFICIENTS 134 3.3.3 PARTIAL MOLAR QUANTITIES 137
3.3.4 PHASE EQUILIBRIA 145 3.4 CHEMICAL KINETICS AS A TEST FOR CHEMICAL
MODELS ON THE MM LEVEL . 149 3.4.1 PRIMARY KINETIC SALT EFFECT 151 3.4.2
SOLVENT EFFECTS 153 3.4.3 SUBSTITUENT EFFECTS 155 3.4.4 REACTIVITY OF
ION PAIRS IN CHEMICAL REACTIONS 156 3.5 TRANSPORT EQUATIONS ON THE LCCM
LEVEL 157 3.5.1 HYDRODYNAMIC ION-ION INTERACTIONS 157 3.5.2
ELECTROPHORETIC TRANSPORT AND CHEMICAL REACTIONS 158 3.5.3
ELECTROPHORETIC TERM OF THE CONDUCTIVITY EQUATION 161 3.5.4 LIMITING LAW
OF CONDUCTIVITY 162 3.5.5 CONDUCTIVITY EQUATIONS FOR SYMMETRICAL
ELECTROLYTES ON THE LCCM LEVEL 164 3.5.6 TRANSFERENCE NUMBERS AND SINGLE
ION CONDUCTIVITIES 169 3.5.7 UNSYMMETRICAL ELECTROLYTES AND ELECTROLYTE
MIXTURES 171 3.5.8 DIFFUSION COEFFICIENTS 172 3.5.9 VISCOSITY 177
REFERENCES 178 CONTENTS XV 4 TOWARDS HIGHER CONCENTRATIONS: THE
DESCRIPTION OF EQUILIBRIUM PROPERTIES 183 4.1 ENSEMBLES 184 4.2 THE
CLASSICAL LIMIT 186 4.2.1 DISTRIBUTION FUNCTIONS OF THE CANONICAL
ENSEMBLE 186 4.2.2 BBGKY HIERARCHY 188 4.2.3 DISTRIBUTION FUNCTIONS OF
THE GRAND CANONICAL ENSEMBLE 189 4.2.4 THERMODYNAMIC FUNCTIONS 190 4.3
CLUSTER EXPANSIONS OF CORRELATION FUNCTIONS 192 4.3.1 PAIR CORRELATION
FUNCTION 192 4.3.2 VIRIAL EQUATION OF PRESSURE 196 4.4 INTEGRAL EQUATION
THEORIES 198 4.4.1 ORNSTEIN-ZERNIKE EQUATION 198 4.4.2 INTEGRAL
EQUATIONS 200 4.5 COULOMBIC SYSTEMS 203 4.5.1 LOCAL ELECTRONEUTRALITY
203 4.5.2 LOW CONCENTRATION LIMIT 206 4.6 INTEGRAL EQUATIONS FOR
ELECTROLYTE SOLUTIONS ON THE MM LEVEL .... 207 4.6.1 MCMILLAN-MAYER
THEOREM 207 4.6.2 FROM THE DEBYE-HIICKEL EQUATION TO INTEGRAL EQUATIONS:
CLUSTER EXPANSIONS 209 4.6.3 CLOSURE RELATIONS FOR INTEGRAL EQUATIONS
211 4.7 HNC RESULTS ON THE MM LEVEL 212 4.8 MSA RESULTS ON THE MM LEVEL
216 4.8.1 PY THERMODYNAMICS FOR HARD SPHERE SYSTEMS IN THE RPM 217 4.8.2
WIENER-HOPF FACTORIZATION 220 4.8.3 CHARGED HARD SPHERES IN THE MSA 221
4.8.4 MSA FOR ARBITRARY CHARGES AND RADII 225 4.8.5 MSA MODELS OF ION
ASSOCIATION 229 4.8.6 SOME MSA APPROACHES FOR ENGINEERS 236 4.9 PAIR
CORRELATION FUNCTIONS INFERRED FROM STATIC STRUCTURE FACTORS . . . 237
4.9.1 STATIC STRUCTURE FACTOR 238 4.9.2 NEUTRON SCATTERING EXPERIMENTS
241 4.9.3 X-RAY EXPERIMENTS 254 4.10 PARTICULAR TECHNIQUES TO VERIFY
MODEL PAIR CORRELATION FUNCTIONS 259 REFERENCES 260 5 REFINED
ELECTROLYTE THEORY: MODELS ON THE BO LEVEL 263 5.1 COMPUTER SIMULATIONS
264 5.2 CLASSICAL SYSTEMS WITH LONG-RANGE FORCES ON THE BO LEVEL 270
5.2.1 GENERALIZED VIRIAL EXPANSIONS AND INTEGRAL EQUATIONS FOR
CORRELATION FUNCTIONS 270 5.2.2 THERMODYNAMIC FUNCTIONS 274 5.3 IONS IN
APOLAR SOLVENTS 276 XVI CONTENTS 5.4 MOLECULAR CORRELATION FUNCTIONS FOR
SYSTEMS WITH ANISOTROPIC INTERACTIONS: INVARIANT EXPANSIONS 279 5.5
SIMPLE MODELS FOR ELECTROLYTE SOLUTIONS: MIXTURES OF CHARGED AND DIPOLAR
HARD SPHERES 281 5.5.1 HARD SPHERES WITH POINT DIPOLES: MSA 281 5.5.2
THE LIN APPROXIMATION FOR DIPOLAR HARD SPHERES 286 5.5.3 POLARIZABILITY
OF SOLVENT MOLECULES 288 5.5.4 HARD SPHERES WITH POINT DIPOLES: HNC AND
RHNC APPROXIMATIONS 289 5.5.5 MIXTURES OF CHARGED AND DIPOLAR HARD
SPHERES IN THE MSA 291 5.6 MOLECULAR MODELS FOR IONS AND SOLVENT:
NUMERICAL SOLUTIONS 299 5.6.1 INTERACTION SITE MODELS 299 5.6.2 THE
SITE-SITE ORNSTEIN ZERNIKE (SSOZ) EQUATION 301 5.6.3 COMPARISON OF
INTEGRAL EQUATION APPROACHES AND COMPUTER SIMULATIONS 303 5.7 ION
SOLVATION IN THE BO AND MM APPROACHES 308 5.7.1 ENERGY OF SOLVATION AND
DIELECTRIC POLARIZATION OF MIXTURES MADE UP OF CHARGED HARD SPHERES AND
DIPOLAR HARD SPHERES 308 5.7.2 POTENTIAL OF MEAN FORCE AT INFINITE
DILUTION 311 5.8 THE CONNECTION BETWEEN BO AND MM DESCRIPTIONS 316 5.9
FURTHER DEVELOPMENTS 317 REFERENCES 317 6 DYNAMICAL AND TRANSPORT
PROPERTIES AT MOLAR CONCENTRATIONS . . . 321 6.1 INTRODUCTION 321 6.2
THE BORN-OPPENHEIMER LEVEL 324 6.2.1 PRINCIPLE OF MOLECULAR DYNAMICS 324
6.2.2 EXPERIMENTAL AND MODEL APPROACHES 326 6.3 LANGEVIN DYNAMICS 333
6.4 SMOLUCHOWSKI DYNAMICS 339 6.4.1 CHARACTERISTIC TIMES 339 6.4.2
SMOLUCHOWSKY DYNAMICS (SD) SIMULATIONS 339 6.4.3
ALTENBERGER-ZHONG-FRIEDMAN (AZF) THEORY 341 6.5 THE CONTINUITY EQUATION
APPROACH 345 6.5.1 BASIC EQUATIONS 345 6.5.2 LOW CONCENTRATION CHEMICAL
MODEL OF ION TRANSPORT 349 6.5.3 MSA AND HNC APPROACHES TO IONIC
TRANSPORT 349 6.5.4 NON-EQUILIBRIUM OZ EQUATION: THE CONCEPT OF THE
DIRECT CORRELATION FORCE 358 REFERENCES 371 7 APPENDIX 373 7.1 PHYSICAL
PROPERTIES AND EMPIRICAL PARAMETERS OF WATER AND ORGANIC SOLVENTS 373
7.1.1 PHYSICAL PROPERTIES 373 7.1.2 EMPIRICAL PARAMETERS 373 CONTENTS
XVII 7.2 LIMITING ION CONDUCTIVITIES OF ELECTROLYTE SOLUTIONS 379 7.3
SOLVENT AND SOLUTION PERMITTIVITIES OF ELECTROLYTE SOLUTIONS 381 7.4
PITZER PARAMETERS FOR OSMOTIC PRESSURE OF NON-AQUEOUS ELECTROLYTE
SOLUTIONS 386 7.5 SYMBOLS AND ABBREVIATIONS 388 REFERENCES 392 SUBJECT
INDEX 395 I
|
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| illustrated | Illustrated |
| indexdate | 2024-12-20T10:19:56Z |
| institution | BVB |
| isbn | 3798510768 |
| language | German |
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| physical | XVII, 401 S. graph. Darst. |
| publishDate | 1998 |
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| publishDateSort | 1998 |
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| series | Topics in physical chemistry |
| series2 | Topics in physical chemistry |
| spellingShingle | Barthel, Josef 1929- Krienke, Hartmut Kunz, Werner 1960- Physical chemistry of electrolyte solutions modern aspects Topics in physical chemistry Elektrolytlösung (DE-588)4133913-7 gnd |
| subject_GND | (DE-588)4133913-7 (DE-588)4143413-4 |
| title | Physical chemistry of electrolyte solutions modern aspects |
| title_auth | Physical chemistry of electrolyte solutions modern aspects |
| title_exact_search | Physical chemistry of electrolyte solutions modern aspects |
| title_full | Physical chemistry of electrolyte solutions modern aspects J. M. G. Barthel ; H. Krienke ; W. Kunz. [Ed. by Deutsche Bunsen-Gesellschaft für physikalische Chemie e.V.] |
| title_fullStr | Physical chemistry of electrolyte solutions modern aspects J. M. G. Barthel ; H. Krienke ; W. Kunz. [Ed. by Deutsche Bunsen-Gesellschaft für physikalische Chemie e.V.] |
| title_full_unstemmed | Physical chemistry of electrolyte solutions modern aspects J. M. G. Barthel ; H. Krienke ; W. Kunz. [Ed. by Deutsche Bunsen-Gesellschaft für physikalische Chemie e.V.] |
| title_short | Physical chemistry of electrolyte solutions |
| title_sort | physical chemistry of electrolyte solutions modern aspects |
| title_sub | modern aspects |
| topic | Elektrolytlösung (DE-588)4133913-7 gnd |
| topic_facet | Elektrolytlösung Aufsatzsammlung |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=008003362&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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