Verfügbarkeit: Optical properties of metal clusters | Technische Universität München

Optical properties of metal clusters:

Gespeichert in:

Bibliographische Detailangaben
Beteiligte Personen:	Kreibig, Uwe (VerfasserIn), Vollmer, Michael (VerfasserIn)
Format:	Buch
Sprache:	Deutsch
Veröffentlicht:	Berlin u.a. Springer 1995
Schriftenreihe:	Springer series in materials science 25
Schlagwörter:	Electronic structure Metal clusters > Optical properties Optische Eigenschaft Metallcluster
Links:	http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=006557118&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA
Beschreibung:	Hier auch später erschienene, unveränderte Nachdrucke
Umfang:	XX, 532 S. Ill., graph. Darst.
ISBN:	3540578366 0387578366 9783642081910

Internformat

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Datensatz im Suchindex

DE-BY-TUM_call_number	0202 PHY 546f 2002 A 4154 0302 CHE 315f 1995 A 5393
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adam_text	UWE KREIBIG MICHAEL VOLLMER OPTICAL PROPERTIES OF METAL CLUSTERS WITH 236 FIGURES SPRINGER TABLE OF CONTENTS 1. INTRODUCTION 1 2. THEORETICAL CONSIDERATIONS 13 2.1 SINGLE CLUSTERS: EXTRINSIC SIZE EFFECTS OF THE OPTICAL PROPERTIES . 14 2.1.1 OPTICAL MATERIAL FUNCTIONS OF BULK METALS 14 (A) FREE ELECTRON OPTICAL RESPONSE 14 (B) INTERBAND TRANSITIONS AND CORE EFFECTS IN REALISTIC METALS 16 (C) FUNDAMENTAL PROPERTIES OF THE DIELECTRIC FUNCTION ... 19 (D) PENETRATION DEPTH OF ELECTROMAGNETIC WAVES IN METALS 21 2.1.2 QUASISTATIC RESPONSE OF A SMALL METAL SPHERE TO AN ELECTRIC FIELD 23 2.1.3 EXACT ELECTRODYNAMIC CALCULATION OF SPHERICAL METAL CLUSTERS (MIE THEORY) 26 (A) RESPONSE OF METAL SPHERES 28 (B) POSITIONS AND SHAPES OF PLASMA RESONANCES 30 (C) RESONANCES OF SPECIAL METALS 35 (D) EXTRINSIC CLUSTER SIZE EFFECTS 41 2.1.4 EXTENSIONS OF THE MIE THEORY 53 (A) NONSPHERICAL CLUSTER SHAPES 54 (B) CORE-SHELL PARTICLES (SPHERICAL HETERO-SYSTEMS) 58 (C) SUBSTRATE EFFECTS 61 (D) NEAR FIELDS AND SURFACE ENHANCED RAMAN SCATTERING 63 (E) NONLINEAR OPTICAL EFFECTS 69 (F) NONLOCAL RESPONSE AND ADDITIONAL SURFACE ABSORPTION 72 (G) LONGITUDINAL PLASMONS 75 2.2 SINGLE CLUSTERS: INTRINSIC SIZE EFFECTS OF THE OPTICAL PROPERTIES . 76 2.2.1 SIZE-DEPENDENT OPTICAL MATERIAL FUNCTIONS OF METAL CLUSTERS 78 (A) GENERAL REMARKS 78 (B) CLASSICAL MODELS FOR E(W, R) 79 (C) QUANTUM-MECHANICAL MODELS FOR E(U , R) 88 2.2.2 DIRECT QUANTUM-MECHANICAL CALCULATIONS OF THE OPTICAL RESPONSE 99 X TABLE OF CONTENTS (A) JELLIUM APPROXIMATION METHODS 101 (B) QUANTUM CHEMICAL METHODS 108 (C) WIDTHS AND SHAPES OF THE RESONANCES 114 2.2.3 EFFECTS OF LOWER-LYING ELECTRONS 118 2.3 CLUSTER MATTER 123 2.3.1 CLASSIFICATION OF CLUSTER MATTER 124 (A) TOPOLOGICAL AND OPTICAL CHARACTERISTICS OF CLUSTER MATTER 124 (B) THE EFFECTIVE FIELD 133 2.3.2 STATISTICALLY DISTRIBUTED SINGLE CLUSTERS: EFFECTIVE MEDIUM THEORIES 135 (A) SURVEY OF EFFECTIVE MEDIUM CONCEPTS 137 (B) DERIVATION OF THE GENZEL E E FF 147 (C) BOUNDS OF E FF 150 (D) CLUSTER SIZE LIMITATIONS 152 (E) EFFECTIVE MEDIA WITH OPTICALLY NONLINEAR CLUSTERS OR MATRICES 152 2.3.3 SEPARATED CLUSTER AGGREGATES: QUASI-STATIC AND ELECTRODYNAMIC CALCULATIONS 155 (A) QUASI-STATIC APPROXIMATION 157 (B) THE CLUSTER PAIR 158 (C) THE LINEAR CLUSTER TRIPLET AND LINEAR CLUSTER CHAINS 160 (D) DIPOLE COUPLING IN SINGLE EXTENDED CLUSTER ARRAYS . . 161 (E) THE GENERAL CASE: GENERALIZED MIE THEORY (GMT) . . 164 2.3.4 DENSELY PACKED MIXTURES OF CLUSTERS AND AGGREGATES .... 171 (A) COMBINATION OF SEPARATED SINGLE CLUSTERS AND AGGREGATES 172 (B) OTHER STATISTICAL CONCEPTS 174 (C) THE BERGMAN EFFECTIVE DIELECTRIC FUNCTION 177 2.3.5 NANOSTRUCTURED MATTER 184 2.4 SUMMARY AND DISCUSSION 187 2.4.1 LARGE CLUSTERS: SURFACE PLASMONS 187 2.4.2 SMALL AND VERY SMALL CLUSTERS: WHAT IS A PLASMON? .... 193 3. EXPERIMENTAL METHODS 203 3.1 GENERAL REMARKS 203 3.2 PREPARATION OF METAL CLUSTERS 207 3.2.1 GENERAL REMARKS 208 3.2.2 FREE CLUSTERS 212 3.2.3 CLUSTERS ON SURFACES 214 3.2.4 CLUSTERS IN SOLIDS 216 (A) MATRIX ISOLATION, COLOR CENTERS, PHOTOGRAPHIC MATERIALS 216 (B) GLASSES AND POLYMERS 218 TABLE OF CONTENTS XI (C) OTHER METHODS 219 3.2.5 CLUSTERS IN LIQUIDS 220 3.2.6 LIGAND STABILIZED CLUSTERS 226 3.2.7 CLUSTER AGGREGATES 231 (A) COAGULATION AGGREGATES 231 (B) COALESCENCE AGGREGATES 232 3.2.8 DENSE CLUSTER MATTER 233 3.3 CHARACTERIZATION OF METAL CLUSTERS 234 3.3.1 GENERAL REMARKS 235 3.3.2 CLUSTERS IN BEAMS 236 3.3.3 CLUSTERS ON SUPPORTS, IN MATRICES ETC 238 (A) TRANSMISSION ELECTRON MICROSCOPY 238 (B) ELECTRON DIFFRACTION 245 (C) OTHER METHODS 246 (D) CLUSTER MATTER 250 3.4 NONDESTRUCTIVE SPECTROSCOPIES 255 3.4.1 COMMON METHODS 255 3.4.2 OTHER TECHNIQUES 259 3.4.3 EXPERIMENTAL MEASURES FOR ABSORPTION, SCATTERING, AND EXTINCTION 260 3.4.4 ADVANTAGES AND DRAWBACKS 265 3.5 DESTRUCTIVE SPECTROSCOPIES 266 3.5.1 TWO PHOTON IONIZATION 267 3.5.2 BEAM DEPLETION SPECTROSCOPY 270 3.5.3 DISSOCIATION SPECTROSCOPY OF SUPPORTED CLUSTERS 272 3.5.4 ADVANTAGES AND DRAWBACKS 273 4. EXPERIMENTAL RESULTS AND DISCUSSION 275 4.1 LARGE CLUSTERS 278 4.1.1 LARGE CLUSTERS IN BEAMS AND SMOKE 278 (A) SMOKES 278 (B) BEAMS 281 (C) INCANDESCENT RADIATION FROM CLUSTERS 284 4.1.2 SEPARATED LARGE CLUSTERS IN MATRICES 285 (A) GENERAL REMARKS 285 (B) EXPERIMENTAL VERIFICATION OF MIE S THEORY 286 (C) MIE DIPOLE RESONANCE: POSITION, WIDTH, THE 1/FI-EFFECT, AND CHEMICAL INTERFACE DAMPING (CID) 294 (D) SPHERICAL CLUSTERS IN VARIOUS MATRICES 302 (E) ELLIPSOIDAL CLUSTERS 305 (F) THE DIELECTRIC FUNCTION OF CLUSTER MATERIAL AND STRUCTURAL PHASE TRANSITIONS 307 XII TABLE OF CONTENTS (G) SIZE EFFECTS IN THE TEMPERATURE DEPENDENCE OF THE CLUSTER ABSORPTION 317 4.1.3 LARGE CLUSTERS ON SUPPORTS 321 (A) THIN FILMS 322 (B) VERIFICATION OF THEORETICAL APPROACHES 323 (C) SHAPE AND SUBSTRATE EFFECTS 324 (D) SURFACE PLASMON INDUCED DESORPTION 328 4.2 SMALL AND VERY SMALL CLUSTERS 333 4.2.1 SMALL AND VERY SMALL FREE CLUSTERS IN BEAMS 333 (A) TRIMERS 333 (B) VERY SMALL CLUSTERS 334 (C) BETWEEN SMALL AND LARGE CLUSTERS 342 (D) PICO- AND FEMTOSECOND SPECTROSCOPY 349 4.2.2 SMALL AND VERY SMALL CLUSTERS IN MATRICES 351 (A) EXPERIMENTS CONCERNING PHOTOGRAPHY 352 (B) CHEMICALLY PREPARED LIGAND STABILIZED CLUSTERS 353 (C) PHYSICALLY PREPARED CLUSTERS 358 4.2.3 SMALL AND VERY SMALL CLUSTERS ON SURFACES 364 (A) ISLAND FILMS 364 (B) FROM VERY SMALL TO SMALL SPHERES AND ELLIPSOIDS.... 364 4.3 SPECIAL EXPERIMENTS 366 4.3.1 FROM MOLECULAR TO METALLIC CLUSTERS: COVERING ALL SIZE RANGES 366 4.3.2 HETEROGENEOUS CLUSTERS 371 (A) BINARY AG/AU SYSTEMS: NUCLEUS/SHELL AND HOMOGENEOUS ALLOY CLUSTERS 372 (B) DIELECTRIC CORE CLUSTERS 374 (C) OTHER SHELL CLUSTERS 375 4.3.3 SERS FROM CLUSTER SAMPLES 376 4.3.4 CHEMICAL REACTIONS 380 (A) GENERAL REMARKS 380 (B) EXPERIMENTS 382 (C) CONCLUSIONS 386 4.3.5 NONLINEAR OPTICAL EFFECTS OF CLUSTERS 387 (A) SECOND ORDER PROCESSES 387 (B) THIRD ORDER PROCESSES 388 4.3.6 LIGHT EMISSION BY NONOPTICAL EXCITATION 389 (A) ELECTROLUMINESCENCE 391 (B) EXCITATION WITH FAST ELECTRONS 393 (C) EXCITATION WITH TUNNELING ELECTRONS 393 4.4 CLUSTER MATTER 395 4.4.1 INTERACTING SINGLE CLUSTERS AND AGGREGATES 397 (A) COMPARISON TO EFFECTIVE MEDIUM THEORIES 397 (B) HIGHER ORDER EXTINCTION PROCESSES 403 TABLE OF CONTENTS XIII (C) COAGULATION EFFECTS 407 (D) QUANTITATIVE COMPARISON TO DIRECT ELECTRODYNAMIC CALCULATIONS 413 (E) LIGHT-INDUCED AGGREGATION 418 4.4.2 COALESCENCE EFFECTS 420 4.4.3 DENSE CLUSTER MATTER 425 (A) THE OSEEN TRANSITION 425 (B) TRANSITION TO COMPACT THIN FILMS 432 APPENDIX 437 A.L TABLES: OPTICAL SPECTROSCOPY EXPERIMENTS WITH METAL CLUSTERS 437 A.2 SURVEY OF OPTICAL SPECTRA OF ELEMENTAL METAL CLUSTERS AND CHAIN-AGGREGATES 451 A.3 MIE COMPUTER PROGRAM 473 REFERENCES J 483 SUBJECT INDEX 527
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language	German
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physical	XX, 532 S. Ill., graph. Darst.
publishDate	1995
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publisher	Springer
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series	Springer series in materials science
series2	Springer series in materials science
spellingShingle	Kreibig, Uwe Vollmer, Michael Optical properties of metal clusters Springer series in materials science Electronic structure Metal clusters Optical properties Optische Eigenschaft (DE-588)4123887-4 gnd Metallcluster (DE-588)4128942-0 gnd
subject_GND	(DE-588)4123887-4 (DE-588)4128942-0
title	Optical properties of metal clusters
title_auth	Optical properties of metal clusters
title_exact_search	Optical properties of metal clusters
title_full	Optical properties of metal clusters Uwe Kreibig ; Michael Vollmer
title_fullStr	Optical properties of metal clusters Uwe Kreibig ; Michael Vollmer
title_full_unstemmed	Optical properties of metal clusters Uwe Kreibig ; Michael Vollmer
title_short	Optical properties of metal clusters
title_sort	optical properties of metal clusters
topic	Electronic structure Metal clusters Optical properties Optische Eigenschaft (DE-588)4123887-4 gnd Metallcluster (DE-588)4128942-0 gnd
topic_facet	Electronic structure Metal clusters Optical properties Optische Eigenschaft Metallcluster
url	http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=006557118&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA
volume_link	(DE-604)BV000683335
work_keys_str_mv	AT kreibiguwe opticalpropertiesofmetalclusters AT vollmermichael opticalpropertiesofmetalclusters

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