Verfügbarkeit: High temperature polymer electrolyte membrane fuel cells

High temperature polymer electrolyte membrane fuel cells: modeling, simulation, and segmented measurements

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Bibliographische Detailangaben
Beteilige Person:	Siegel, Christian (VerfasserIn)
Format:	Hochschulschrift/Dissertation Buch
Sprache:	Englisch
Veröffentlicht:	Berlin Logos Verlag Berlin GmbH [2015]
Schlagwörter:	Betriebsverhalten Membranelektrode Polymer-Elektrolytmembran-Brennstoffzelle Finite-Elemente-Methode Dreidimensionale Strömung Hochtemperaturbrennstoffzelle Phosphorsäure Numerische Strömungssimulation Polybenzimidazole Hochschulschrift
Links:	http://deposit.dnb.de/cgi-bin/dokserv?id=5179418&prov=M&dok_var=1&dok_ext=htm http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030101294&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA
Umfang:	XVI, 161 Seiten Illustrationen, Diagramme 24 cm
ISBN:	9783832539177 3832539174

Internformat

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Datensatz im Suchindex

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adam_text	TABLE OF CONTENT ABSTRACT I ZUSAMMENFASSUNG ID ACKNOWLEDGMENTS V TABLE OF CONTENT VII NOMENCLATURE XI 1. INTRODUCTION 1 2. FUEL CELLS 3 2.1 WORKING PRINCIPLE 4 2.2 HTPEM FUEL CELLS 5 2.3PBI/H 3 P0 4 MEA 6 2.4 OVERALL FEATURES OF A PBI/H3PO4 MEA 6 2.5 FUTURE DEVELOPMENT 8 2.6 FUEL CELL THERMODYNAMICS 8 2.6.1 POTENTIAL OF A FUEL CELL 8 2.6.2 EFFICIENCY OF A FUEL CELL 12 2.7 FUEL CELL CHARACTERIZATION METHODS 13 2.7.1 CURRENT-VOLTAGE-CURVE (I-V-CURVE) OF A PEM FUEL CELL 13 2.7.2 ELECTROCHEMICAL IMPEDANCE SPECTROSCOPY 15 3. PEM FUEL CELL MODELING 19 3.1 OVERALL MODELING ASPECTS 20 3.2 HTPEM FUEL CELL MODELS - LITERATURE REVIEW 21 4. THE DEVELOPED HTPEM FUEL CELL MODEL 23 4.1 MODEL GEOMETRY 23 4.1.1 TYPE I FLOW-FIELD 25 4.1.2 TYPE 0 FLOW-FIELD 25 4.1.3 TYPE III FLOW-FIELD 25 4.2 SUBDOMAIN TRANSPORT EQUATIONS 26 4.2.1 MOMENTUM TRANSPORT 26 4.2.2 MASS (SPECIES) TRANSPORT 27 4.2.3 ENERGY TRANSPORT 27 4.2.4 CHARGE TRANSPORT 28 4.2.5 ELECTROCHEMISTRY AND TRANSPORT PROPERTIES FOR THE SPHERICAL AGGLOMERATE MODEL 29 4.2.6 KINETIC PARAMETERS AND TRANSPORT PROPERTIES IN PHOSPHORIC ACID 33 4.2.7 PBI/H3PO4 SOL-GEL MEMBRANE MODELING 37 VII HTTP://D-NB.INFO/1068597690 4.2.8 FLUID-(GAS)-, AND SOLID-PHASE PROPERTIES AND MATERIAL CORRELATIONS 38 4.3 BOUNDARY CONDITIONS 40 4.4 INITIAL CONDITIONS 42 4.6 ASSUMPTIONS AND SIMPLIFICATIONS 43 4.6 MODELING PARAMETERS 44 5. SOLVING THE MODEL 47 5.1 MESHING 47 5.2 SOLUTION PROCEDURE AND CONVERGENCE BEHAVIOUR 50 6. THE SEGMENTED HTPEM FUEL CELL 53 6.1 SEGMENTED MEASUREMENTS - LITERATURE REVIEW 53 6.1.1 TEMPERATURE MEASUREMENTS 53 6.1.2 CURRENT DENSITY MEASUREMENTS 54 6.1.3 E1S MEASUREMENTS 54 6.2 REQUIREMENTS, MANUFACTURING AND ASSEMBLING 57 6.3 MEASURING THE SOLID-PHASE TEMPERATURE DISTRIBUTION 60 6.4 MEASURING THE CURRENT DENSITY DISTRIBUTION 60 6.5 SEGMENTED EIS MEASUREMENTS 61 6.5.1 THE SIMPLIFIED SET-UP FOR SEGMENTED EIS MEASUREMENTS 61 6.5.2 NOTE ON THE EXPERIMENTAL SET-UP 62 6.6 EQUIVALENT CIRCUIT MODELING 63 6.7 ANALYSIS OF THE EIS DATA 64 6.8 OPERATING THE NONSEGMENTED AND SEGMENTED HTPEM FUEL CELL 65 7. CHARACTERIZING THE THREE TYPES OF FLOW-FIELDS 67 7.1 FLUID-FLOW DISTRIBUTION AND PRESSURE DROP 67 7.1.1 TYPE I FLOW-FIELD 67 7.1.2 TYPE II FLOW-FIELD 69 7.1.3 TYPE III FLOW-FIELD 70 7.2 IMPEDANCE MEASUREMENTS AT NO-LOAD OPERATING CONDITIONS 72 7.3 OVERALL PERFORMANCE AT REFERENCE OPERATING CONDITIONS 73 7.3.1 TYPE I FLOW-FIELD 74 7.3.2 TYPE II FLOW-FIELD 75 7.3.3 TYPE III FLOW-FIELD 76 8. SEGMENTED SOLID-PHASE TEMPERATURE AND CURRENT DENSITY MEASUREMENTS 77 8.1 SOLID-PHASE TEMPERATURE DISTRIBUTION AT NO-LOAD OPERATING CONDITIONS 77 8.1.1 TYPE I FLOW-FIELD 77 8.1.2 TYPE II FLOW-FIELD 80 VIII 8.1.3 TYPE III FLOW-FIELD 83 8.2 LOAD OPERATING CONDITIONS - COUNTER-FLOW CONFIGURATION 86 8.2.1 TYPE I FLOW-FIELD - OPERATION WITH HYDROGEN AND AIR 86 8.2.2 TYPE I FLOW-FIELD - OPERATION WITH CO ENRICHED HYDROGEN AND AIR 95 8.2.3 TYPE N FLOW-FIELD - OPERATION WITH HYDROGEN AND AIR 97 8.2.4 TYPE II FLOW-FIELD - OPERATION WITH CO ENRICHED HYDROGEN AND AIR 105 8.2.5 TYPE III FLOW-FIELD-OPERATION WITH HYDROGEN AND AIR 108 8.2.6 TYPE III FLOW-FIELD - OPERATION WITH CO ENRICHED HYDROGEN AND AIR 115 8.3 LOAD OPERATING CONDITIONS - CO-FLOW CONFIGURATION 116 8.3.1 TYPE I FLOW-FIELD - OPERATION WITH HYDROGEN AND AIR 116 8.3.2 TYPE I FLOW-FIELD - OPERATION WITH CO ENRICHED HYDROGEN AND AIR 118 8.3.3 TYPE II FLOW-FIELD - OPERATION WITH HYDROGEN AND AIR 120 8.3.4 TYPE II FLOW-FIELD - OPERATION WITH CO ENRICHED HYDROGEN AND AIR 123 8.3.5 TYPE III FLOW-FIELD - OPERATION WITH HYDROGEN AND AIR 123 8.3.6 TYPE III FLOW-FIELD - OPERATION WITH CO ENRICHED HYDROGEN AND AIR 125 9. SEGMENTED EIS MEASUREMENTS IN A HTPEM FUEL CELL 129 9.1 TYPE I FLOW-FIELD 129 9.2 TYPE II FLOW-FIELD 131 9.3 TYPE III FLOW-FIELD 137 10. CONCLUSION 143 10.1 MODELING AND SIMULATION 143 10.2 EXPERIMENTAL 144 10.3 SOLID-PHASE TEMPERATURE DISTRIBUTION 144 10.4 CURRENT DENSITY DISTRIBUTION 146 10.5 SEGMENTED EIS MEASUREMENTS 147 11. REFERENCES 149 IX
any_adam_object	1
author	Siegel, Christian
author_facet	Siegel, Christian
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author_variant	c s cs
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dewey-raw	621.312429
dewey-search	621.312429
dewey-sort	3621.312429
dewey-tens	620 - Engineering and allied operations
discipline	Chemie / Pharmazie Elektrotechnik / Elektronik / Nachrichtentechnik Energietechnik
format	Thesis Book
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spellingShingle	Siegel, Christian High temperature polymer electrolyte membrane fuel cells modeling, simulation, and segmented measurements Betriebsverhalten (DE-588)4138142-7 gnd Membranelektrode (DE-588)4169393-0 gnd Polymer-Elektrolytmembran-Brennstoffzelle (DE-588)4450903-0 gnd Finite-Elemente-Methode (DE-588)4017233-8 gnd Dreidimensionale Strömung (DE-588)4150635-2 gnd Hochtemperaturbrennstoffzelle (DE-588)4160270-5 gnd Phosphorsäure (DE-588)4174437-8 gnd Numerische Strömungssimulation (DE-588)4690080-9 gnd Polybenzimidazole (DE-588)7847092-4 gnd
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title	High temperature polymer electrolyte membrane fuel cells modeling, simulation, and segmented measurements
title_auth	High temperature polymer electrolyte membrane fuel cells modeling, simulation, and segmented measurements
title_exact_search	High temperature polymer electrolyte membrane fuel cells modeling, simulation, and segmented measurements
title_full	High temperature polymer electrolyte membrane fuel cells modeling, simulation, and segmented measurements von Christian Siegel aus Mondercange, Luxemburg
title_fullStr	High temperature polymer electrolyte membrane fuel cells modeling, simulation, and segmented measurements von Christian Siegel aus Mondercange, Luxemburg
title_full_unstemmed	High temperature polymer electrolyte membrane fuel cells modeling, simulation, and segmented measurements von Christian Siegel aus Mondercange, Luxemburg
title_short	High temperature polymer electrolyte membrane fuel cells
title_sort	high temperature polymer electrolyte membrane fuel cells modeling simulation and segmented measurements
title_sub	modeling, simulation, and segmented measurements
topic	Betriebsverhalten (DE-588)4138142-7 gnd Membranelektrode (DE-588)4169393-0 gnd Polymer-Elektrolytmembran-Brennstoffzelle (DE-588)4450903-0 gnd Finite-Elemente-Methode (DE-588)4017233-8 gnd Dreidimensionale Strömung (DE-588)4150635-2 gnd Hochtemperaturbrennstoffzelle (DE-588)4160270-5 gnd Phosphorsäure (DE-588)4174437-8 gnd Numerische Strömungssimulation (DE-588)4690080-9 gnd Polybenzimidazole (DE-588)7847092-4 gnd
topic_facet	Betriebsverhalten Membranelektrode Polymer-Elektrolytmembran-Brennstoffzelle Finite-Elemente-Methode Dreidimensionale Strömung Hochtemperaturbrennstoffzelle Phosphorsäure Numerische Strömungssimulation Polybenzimidazole Hochschulschrift
url	http://deposit.dnb.de/cgi-bin/dokserv?id=5179418&prov=M&dok_var=1&dok_ext=htm http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030101294&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA
work_keys_str_mv	AT siegelchristian hightemperaturepolymerelectrolytemembranefuelcellsmodelingsimulationandsegmentedmeasurements

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