Soil colloids: properties and ion binding
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| Main Author: | |
|---|---|
| Format: | Book |
| Language: | English |
| Published: |
Boca Raton [u.a.]
CRC Press
2014
|
| Series: | Surfactant science series
156 |
| Subjects: | |
| Links: | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=026218614&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| Item Description: | Includes bibliographical references and index |
| Physical Description: | XXVIII, 513 S. |
| ISBN: | 9781439851142 |
Staff View
MARC
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Record in the Search Index
| _version_ | 1819311544077385728 |
|---|---|
| adam_text | Titel: Soil colloids
Autor: Molina, Fernando Víctor
Jahr: 2014
Contents
Preface.....................................................................................................................xxi
List of Common Greek Symbols.........................................................................xxiii
List of Common Symbols......................................................................................xxv
List of Common Acronyms..................................................................................xxvii
PART I Foundations
Chapter 1 Introduction..........................................................................................3
1.1 Soil.............................................................................................3
1.2 Soil Chemistry, Soil Colloids, and Metal Ions..........................3
1.3 Book Contents...........................................................................4
References............................................................................................5
Chapter 2 Colloidal Particles and Colloidal Suspensions..
2.1 Colloidal Particles.....................................................................7
2.2 Soil Colloids............................................................................10
2.3 Colloidal Suspensions: General Properties and
Classification...........................................................................14
2.3.1 Importance of Surface in Colloidal Systems.............17
2.3.2 Surface Energy...........................................................18
2.4 Fundamentals of Interfacial Thermodynamics.......................19
2.4.1 Surface Excesses........................................................19
2.4.2 Gibbs Equation...........................................................21
2.5 Summary.................................................................................24
References..........................................................................................25
Chapter 3 Electrified Interface............................................................................27
3.1 Basic Principles.......................................................................27
3.1.1 Electrochemical Equilibrium.....................................27
3.1.2 Poisson and Poisson-Boltzmann Equations...............29
3.1.2.1 Poisson Equation.........................................29
3.1.2.2 Poisson-Boltzmann Equation.....................29
3.2 Application of the Poisson-Boltzmann Equation...................31
3.2.1 Linearization of the PB Equation and the
Debye-Hiickel Theory...............................................31
3.2.2 Gouy-Chapman Theory.............................................34
xiv Contents
3.2.3 Analytical Solutions for Other Cases.........................37
3.2.3.1 Cylindrical Coordinates..............................37
3.2.3.2 Other Cases.................................................39
3.2.4 Numerical Solutions to the Poisson-Boltzmann
Equation.....................................................................39
3.3 Interfacial Capacitance and the Stern and Grahame
Models.....................................................................................42
3.3.1 Interfacial Capacitance...............................................43
3.3.2 Stern Modification......................................................44
3.3.3 Grahame Modification of the Gouy-Chapman-
Stern Theory...............................................................47
3.4 Beyond the Poisson-Boltzmann Equation..............................49
3.5 Approximate Solutions of the PB Equation............................55
3.6 Summary.................................................................................56
References..........................................................................................56
Chapter 4 Sorption onto Colloidal Particles.......................................................63
4.1 General Concepts....................................................................63
4.2 Sorption Isotherms..................................................................63
4.2.1 Gas Phase Isotherm Types.........................................64
4.2.2 Isotherm Classification for Sorption from Solution ...69
4.3 Physical Nature of Adsorption................................................75
4.3.1 Adsorption from Gas Phase.......................................75
4.3.2 Adsorption from Solution...........................................76
4.3.3 Interaction between a Molecule or Ion and a
Surface........................................................................78
4.3.3.1 Intermolecular Interactions.........................78
4.3.3.2 Interactions with a Macroscopic Particle ...83
4.4 Theory of Adsorption Isotherms.............................................86
4.4.1 Limiting (Henry) Isotherm.........................................86
4.4.2 Ideal Monolayer. Langmuir Isotherm........................86
4.4.3 Competitive and Multisite Langmuir Isotherms........89
4.4.4 Ideal Multilayer (BET) Isotherm................................91
4.4.5 Beyond Ideal Isotherms..............................................94
4.4.6 Adsorption with Interactions: The Fowler-
Guggenheim Isotherm................................................95
4.4.7 Surface Heterogeneity................................................98
4.4.7.1 Sips Distribution Function..........................98
4.4.7.2 Langmuir-Freundlich and Freundlich
Isotherms....................................................99
4.5 Other Isotherm Equations.....................................................100
4.6 Isotherm Comparison and Assignment.................................103
4.7 Summary...............................................................................106
References........................................................................................106
Contents xv
Chapter 5 Surface Charge of Colloidal Particles..............................................Ill
5.1 Contributions to Surface Charge...........................................Ill
5.1.1 Permanent Charge....................................................Ill
5.1.2 Protonic and Intrinsic Charge..................................112
5.1.3 Inner and Outer Sphere Complex Charges...............113
5.1.4 Particle Charge Balance...........................................114
5.1.5 Soil Charge...............................................................115
5.2 Ion Sorption and Surface Charge Development....................116
5.3 Ion Exchange.........................................................................118
5.3.1 Thermodynamics of Ion Exchange: Vanselow
Convention................................................................119
5.3.2 Other Conventions and Selectivity Coefficient
Expressions...............................................................122
5.3.2.1 Kerr Convention........................................122
5.3.2.2 Gaines and Thomas Convention...............122
5.3.2.3 Krishnamoorthy and Overstreet
Convention................................................124
5.3.2.4 Gapon Selectivity Coefficient...................125
5.3.2.5 Cernik et al. Convention...........................125
5.3.2.6 Other Aspects...........................................126
5.3.3 Ion Exchange Analysis and Parameter Computation... 127
5.3.3.1 Argensinger Method.................................127
5.3.3.2 Rothmund-Kornfeld Method...................130
5.3.4 Ion Exchange in Soils...............................................131
5.3.4.1 Examples of Ion Exchange in Soils..........133
5.3.4.2 Ion Preference...........................................135
5.4 Determination of Surface Charge.........................................138
5.4.1 Electrophoretic Methods..........................................138
5.4.2 Titration Methods.....................................................144
5.5 Charge Contributions and Points of Zero Charge.................147
5.5.1 Indifferent Electrolytes.............................................148
5.5.2 Charge in the Presence of Specific Adsorption........151
5.6 Summary...............................................................................153
References........................................................................................154
Chapter 6 Interparticle Interactions and Colloid Stability................................159
6.1 Thermodynamics of Particle-Particle Interaction................159
6.2 van der Waals Particle-Particle Interactions.........................161
6.3 Energies and Forces of Interaction........................................166
6.4 Electrostatic Interactions.......................................................168
6.4.1 Constant Potential Conditions..................................170
6.4.1.1 Linear Approximation: The Hogg-
Healy-Fuerstenau Theory........................170
Contents
6.4.1.2 Identical Particles: Verwey-Overbeek
Results.......................................................171
6.4.1.3 Derjaguin Theory.....................................172
6.4.2 Constant Charge Conditions and Comparison
with Constant Potential............................................174
6.4.3 Charge Regulation....................................................176
6.5 Total Long-Range Interactions..............................................178
6.5.1 Similar Surfaces: Classic DLVO Theory.................178
6.5.2 Dissimilar Particles..................................................182
6.5.3 Colloidal Suspension Stability.................................183
6.6 Beyond DLVO.......................................................................188
6.6.1 DLVO Theory Limitations.......................................188
6.6.2 DLVO Extensions.....................................................190
6.6.3 Alternative Models...................................................191
6.7 Summary...............................................................................192
References........................................................................................193
PART II Soil Components
Chapter 7 Soil Composition and Characterization...........................................201
7.1 General Characteristics.........................................................201
7.1.1 Soil Structure............................................................201
7.1.2 Gas, Liquid, and Solid Soil Phases..........................203
7.1.3 Soil Particles.............................................................205
7.1.4 Soil Solution.............................................................205
7.2 Soil Composition...................................................................207
7.2.1 Soil Minerals............................................................207
7.2.1.1 Primary Minerals.....................................208
7.2.1.2 Secondary Minerals..................................210
7.2.1.3 Structural Elements of Soil Minerals.......211
7.2.2 Soil Organic Matter..................................................212
7.2.2.1 Humic Substances.....................................214
7.2.2.2 Nonhumic Substances...............................215
7.3 X-Ray-Based Characterization Methods...............................218
7.3.1 X-Ray Diffraction.....................................................218
7.3.2 X-Ray Absorption-Based Methods..........................219
7.3.3 X-Ray Fluorescence.................................................224
7.3.4 X-Ray Photoelectron Spectroscopy..........................224
7.4 Other Spectroscopic Methods...............................................227
7.4.1 UV-Visible Molecular Spectrometries.....................227
7.4.2 UV-Visible Atomic Spectrometry...........................228
7.4.3 Infrared Spectroscopy..............................................229
7.4.4 Nuclear Magnetic Resonance...................................232
Contents
7.5 Microscopies..........................................................................237
7.5.1 Optical Microscopy..................................................237
7.5.2 Electron Microscopy................................................237
7.5.3 Atomic Force Microscopy........................................238
7.6 Miscellaneous Methods.........................................................241
7.6.1 Neutron Activation Analysis....................................241
7.6.2 Electrophoretic Separations.....................................242
7.6.3 Field-Flow Fractionation..........................................243
7.6.4 Surface Area Measurement......................................243
7.6.4.1 Physical Methods......................................243
7.6.4.2 Positive Adsorption Methods....................244
7.6.4.3 Negative Adsorption Methods..................248
7.6.5 Thermal Analysis Methods......................................249
7.6.5.1 Differential Thermal Analysis..................249
7.6.5.2 Differential Scanning Calorimetry...........252
7.6.5.3 Thermogravimetry....................................253
7.7 Chemical Characterization....................................................253
7.8 Soil Analysis..........................................................................253
7.9 Summary...............................................................................255
References........................................................................................255
Chapter 8 Silicate-Based Minerals..,...............................................................265
8.1 Structure and Classification of Silicate-Based Minerals.......265
8.2 Kaolin-Serpentine Group (1:1) Clays....................................277
8.3 Low Permanent Charge 2:1 Phyllosilicates: Pyrophyllite-
Talc Group.............................................................................278
8.4 Permanently Charged 2:1 Phyllosilicate Minerals................279
8.4.1 Micas........................................................................279
8.4.2 Vermiculites.............................................................281
8.4.3 Smectites..................................................................282
8.4.4 Chlorites...................................................................283
8.4.5 Interstratified Phyllosilicates....................................285
8.5 Other Aluminosilicate Minerals............................................286
8.5.1 Allophane and Imogolite..........................................286
8.5.2 Palygorskite and Sepiolite........................................287
8.5.3 Zeolites.....................................................................288
8.6 Characterization of Silicate Minerals....................................289
8.6.1 Identification and Crystalline Structure...................289
8.6.2 Ion Exchange............................................................290
8.6.3 Specific Surface Area...............................................291
8.7 Ion Binding to Silicate-Based Minerals................................293
8.8 Summary...............................................................................295
References........................................................................................295
xviii Contents
Chapter 9 Oxide Minerals.................................................................................299
9.1 Silica Minerals.......................................................................299
9.2 Aluminum (Hydr)Oxides.......................................................300
9.3 Iron (Hydr)Oxides.................................................................307
9.4 Manganese Oxides................................................................311
9.5 Titanium and Zirconium Oxide Minerals.............................314
9.5.1 Titanium Oxides.......................................................314
9.5.2 Zirconium Minerals.................................................318
9.6 Characterization of Oxides....................................................318
9.6.1 Identification and Crystalline Structure...................318
9.6.2 Spectroscopic Studies...............................................318
9.6.3 Specific Surface Area and Surface Charge..............321
9.6.4 Miscellaneous Methods............................................323
9.7 Ion Binding to Oxide Minerals..............................................323
9.7.1 Cation Binding.........................................................324
9.7.2 Anion Binding..........................................................328
9.8 Summary...............................................................................332
References........................................................................................332
Chapter 10 Humic Substances............................................................................337
10.1 Nature and Classification of Soil Humic Substances............337
10.2 Extraction of HS....................................................................338
10.2.1 Alkaline Extraction..................................................339
10.2.2 Mild Extradants.......................................................341
10.2.2.1 Na4P207 and Other Neutral Salts..............341
10.2.2.2 Formic Acid (HCOOH)............................341
10.2.2.3 Organic Chelating Agents.........................341
10.2.3 Sequential Extractions..............................................342
10.3 Characterization, Composition, and Structure of HS............342
10.3.1 Elemental Composition............................................342
10.3.2 Molecular Weight and Size Distributions................342
10.3.2.1 Colligative Properties...............................343
10.3.2.2 Light Scattering........................................344
10.3.2.3 Size-Exclusion Chromatography..............345
10.3.2.4 Ultracentrifugation...................................345
10.3.2.5 Viscosimetry.............................................347
10.3.2.6 Microscopic Observation..........................348
10.3.2.7 Other Techniques......................................349
10.3.3 Spectroscopic Methods............................................350
10.3.3.1 Infrared Spectroscopy..............................350
10.3.3.2 Nuclear Magnetic Resonance...................350
10.3.3.3 UV-Visible and Fluorescence
Spectroscopy.............................................352
Contents
10.3.4 Functional Groups and Acid-Base Properties.........359
10.3.4.1 Functional Group Analysis.......................359
10.3.4.2 Structural Studies by Chemical
Degradative Methods................................361
10.3.4.3 Structural Studies by Thermal
Degradation..............................................362
10.3.5 Molecular Structure of HS.......................................364
10.4 Ion Binding to Hs..................................................................370
10.5 Summary...............................................................................373
References........................................................................................373
PART III Ion Binding to Soil Colloids
Chapter 11 Modeling Ion Binding: General Concepts.......................................383
11.1 General Problem....................................................................383
11.1.1 Chemical Modeling..................................................385
11.1.2 Modeling Bases.................................................:......387
11.2 Affinity Spectra.....................................................................388
11.2.1 Discrete Affinity Spectra.........................................389
11.2.1.1 Proton-Binding Equilibrium.....................389
11.2.1.2 Competitive Binding.................................390
11.2.2 Continuous Affinity Spectra....................................391
11.2.2.1 Proton Binding..........................................392
11.2.2.2 Competitive Metal Binding......................393
11.3 Extraction of Affinity Spectra...............................................396
11.3.1 Intrinsic and Conditional Equilibrium Constants.... 397
11.3.2 Semianalytical Methods...........................................397
11.3.3 Modified Least Squares Methods.............................399
11.3.4 Maximum Entropy Formalism.................................405
11.4 Kinetic Aspects.....................................................................406
11.5 Summary...............................................................................408
References........................................................................................408
Chapter 12 Ion Binding to Minerals: Discrete Site Modeling............................415
12.1 Ion Binding to Mineral Components.....................................415
12.2 Generic Surface Description: Classical Electrostatic Models...416
12.2.1 Triple-Layer Model..................................................416
12.2.1.1 Model Statement.......................................416
12.2.1.2 Applications of the Triple-Layer Model ...420
12.2.1.3 Further Advances: Extended
Triple-Layer Model...................................422
xx Contents
12.2.2 Simplified Modeling: Basic Stern and Constant
Capacitance Models.................................................424
12.2.3 Stern Extended or Quad Layer Model......................428
12.3 Detailed Surface Description: CD-MUSIC Model...............430
12.3.1 Model Formulation...................................................430
12.3.2 Application of the CD-MUSIC Model.....................433
12.4 Comparison between Models................................................434
12.5 Application to Charge Regulation between Particles............437
12.6 Summary...............................................................................441
References........................................................................................442
Chapter 13 Ion Binding to Humic Substances: Distributed Site Modeling........447
13.1 Ion Binding to Soil Organic Matter.......................................447
13.2 Affinity Spectra of Humic Substances..................................447
13.2.1 Discrete Affinity Spectra.........................................448
13.2.2 Continuous Affinity Spectra....................................452
13.2.3 Structure-Based Affinity Spectra.............................453
13.3 Electrostatic Modeling of Ion Binding to Humic Particles.... 455
13.3.1 Particle Models.........................................................455
13.3.2 Donnan Phase Models..............................................457
13.4 Models for Ion Binding to Humic Substances.......................460
13.4.1 Windermere Humic Models.....................................460
13.4.2 Stockholm Humic Model.........................................462
13.4.3 NICA-Donnan Model..............................................466
13.4.4 NICA-EPN Model...................................................468
13.4.5 Comparison of the Different Models.......................470
13.5 Summary...............................................................................472
References........................................................................................473
Chapter 14 Ion Binding to Soils..........................................................................479
14.1 State of Soil Components in Natural Soils............................479
14.2 Ion Binding to Several Soil Components..............................480
14.2.1 Additivity Rule.........................................................480
14.2.2 Sorption to Binary and Ternary Component
Systems.....................................................................481
14.2.3 Sorption in Complex Systems and Whole Soils.......485
14.3 Models for Ion Sorption to Soils...........................................490
14.3.1 Assemblage Models..................................................490
14.3.2 Incorporation of HS-Mineral Interaction:
LCD Model..............................................................493
14.4 Summary and Perspectives...................................................495
References........................................................................................496
Index......................................................................................................................501
|
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| id | DE-604.BV041244478 |
| illustrated | Not Illustrated |
| indexdate | 2024-12-20T16:34:05Z |
| institution | BVB |
| isbn | 9781439851142 |
| language | English |
| lccn | 2013005085 |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-026218614 |
| oclc_num | 859225560 |
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| owner | DE-29 |
| owner_facet | DE-29 |
| physical | XXVIII, 513 S. |
| publishDate | 2014 |
| publishDateSearch | 2014 |
| publishDateSort | 2014 |
| publisher | CRC Press |
| record_format | marc |
| series | Surfactant science series |
| series2 | Surfactant science series |
| spellingShingle | Molina, Fernando V. Soil colloids properties and ion binding Surfactant science series Soil colloids Soils Analysis Bodenkolloid (DE-588)4146150-2 gnd |
| subject_GND | (DE-588)4146150-2 |
| title | Soil colloids properties and ion binding |
| title_auth | Soil colloids properties and ion binding |
| title_exact_search | Soil colloids properties and ion binding |
| title_full | Soil colloids properties and ion binding Fernando V. Molina |
| title_fullStr | Soil colloids properties and ion binding Fernando V. Molina |
| title_full_unstemmed | Soil colloids properties and ion binding Fernando V. Molina |
| title_short | Soil colloids |
| title_sort | soil colloids properties and ion binding |
| title_sub | properties and ion binding |
| topic | Soil colloids Soils Analysis Bodenkolloid (DE-588)4146150-2 gnd |
| topic_facet | Soil colloids Soils Analysis Bodenkolloid |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=026218614&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| volume_link | (DE-604)BV001889743 |
| work_keys_str_mv | AT molinafernandov soilcolloidspropertiesandionbinding |